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Register a new userCaloric Determination of the Upper Critical Fields and Anisotropy of NdFeAsO1-xFx Single Crystals
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We present heat capacity measurements of the upper critical fields of single-crystal NdFeAsO1-xFx. In zero-magnetic field a clear step in the heat capacity is observed at Tc = 47K . In fields applied perpendicular to the FeAs-layers the step broadens significantly whereas for the in-plane orientation the field effects are small. This behavior is reminiscent of the CuO2-high-Tc superconductors and is a manifestation of pronounced fluctuation effects. Using an entropy conserving construction we determine the transition temperatures in applied fields and the upper critical field slopes of dHc2,a = -0.72 T/K and dHc2,ab = -3.1 T/K. Zero-temperature coherence lengths of xiab = 3.7 nm and xic = 0.9 nm and a modest superconducting anisotropy of gamma ~ 4 can be deduced in a single-band model.
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Superconductivity of Ca1-xLaxFe2As2 single crystals with various doping level were investigated via electromagnetic measurements for out-plane (H//c) and in-plane (H//ab) directions. Obvious double superconducting transitions, which can survive in magnetic fields up to several Tesla, were observed in the medium-doped (x = 0.13) sample. Two kinds of distinct Hc2 phase diagrams were established for the low superconducting phase with Tc lower than 15 K and the high superconducting phase with Tc of over 40 K, respectively. Both the two kinds of phase diagrams exist in the medium-doped sample. Unusual upward curvature near Tc was observed in Hc2 phase diagrams and analyzed in detail. Temperature dependences of anisotropy for different doping concentrations were obtained and compared. Both superconducting phases manifest extremely large anisotropies, which may originate from the interface or intercalation superconductivity.
The newly discovered iron-based superconductors have stimulated enormous interests in the field of superconductivity. Since the new superconductor is a layered system, the anisotropy is a parameter with the first priority to know. Meanwhile any relevant message about the critical fields (upper critical field and irreversibility line) are essentially important. By using flux method, we have successfully grown the single crystals NdO0.82F0.18FeAs at ambient pressure. Resistive measurements reveal a surprising discovery that the anisotropy Gamma = (mc/mab)^{1/2} is below 5, which is much smaller than the theoretically calculated results. The data measured up to 400 K show a continuing curved feature which prevents a conjectured linear behavior for an unconventional metal. The upper critical fields determined based on the Werthamer-Helfand-Hohenberg formula are H_{c2}^{H||ab}(T=0 K) = 304 T and H_{c2}^{H||c}(T=0 K)=62-70 T, indicating a very encouraging application of the new superconductors.
Optimally-doped La1.85Sr0.15CuO4 single crystals have been investigated by dc and ac magnetic measurements. These crystals have rectangular needle-like shapes with the long needle axis parallel to the crystallographic c axis (c-crystal) or parallel to the basal planes (a-crystal). In both crystals, the temperature dependence of the upper critical fields (HC2) and the surface critical field (HC3) were measured. The H-T phase diagram is presented. Close to TC =35 K, for the c-crystal, {gamma}c = / = 1.80(2), whereas for the a-crystal the {gamma}a = / =4.0(2) obtained, is much higher than the theoretical value 1.69. At low applied dc fields, positive field-cooled branches known as the paramagnetic Meissner effect (PME) are observed, their magnitude is inversely proportional to H. The anisotropic PME is observed in both a- and c-crystals, only when the applied field is along the basal planes. It is speculated that the high {gamma}a and the PME are connected to each other.
Early work on the iron-arsenide compounds supported the view, that a reduced dimensionality might be a necessary prerequisite for high-Tc superconductivity. Later, however, it was found that the zero-temperature upper critical magnetic field, Hc2(0), for the 122 iron pnictides is in fact rather isotropic. Here, we report measurements of the temperature dependence of the electrical resistivity, Gamma(T), in Ba0.5K0.5Fe2As2 and Ba0.68K0.32Fe2As2 single crystals in zero magnetic field and for Ba0.68K0.32Fe2As2 as well in static and pulsed magnetic fields up to 60 T. We find that the resistivity of both compounds in zero field is well described by an exponential term due to inter-sheet umklapp electron-phonon scattering between light electrons around the M point to heavy hole sheets at the Gamma point in reciprocal space. From our data, we construct an H-T phase diagram for the inter-plane (H || c) and in-plane (H || ab) directions for Ba0.68K0.32Fe2As2. Contrary to published data for underdoped 122 FeAs compounds, we find that Hc2(T) is in fact anisotropic in optimally doped samples down to low temperatures. The anisotropy parameter, {gamma} = Habc2/Hcc2, is about 2.2 at Tc. For both field orientations we find a concave curvature of the Hc2 lines with decreasing anisotropy and saturation towards lower temperature. Taking into account Pauli spin paramagnetism we perfectly can describe Hc2(T) and its anisotropy.
We use angle resolved photoemission spectroscopy (ARPES) to study the momentum dependence of the superconducting gap in NdFeAsO1-xFx single crystals. We find that the Gamma hole pocket is fully gapped below the superconducting transition temperature. The value of the superconducting gap is 15 +- 1.5 meV and its anisotropy around the hole pocket is smaller than 20% of this value. This is consistent with an isotropic or anisotropic s-wave symmetry of the order parameter or exotic d-wave symmetry with nodes located off the Fermi surface sheets. This is a significant departure from the situation in the cuprates, pointing to possibility that the superconductivity in the iron arsenic based system arises from a different mechanism.
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