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Register a new userFermi Surface and Band Renormalization in (Sr,K)Fe$_2$As$_2$ Superconductor from Angle-Resolved Photoemission Spectroscopy
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High resolution angle-resolved photoemission measurements have been carried out on (Sr,K)Fe$_2$As$_2$ superconductor (Tc=21 K). Three hole-like Fermi surface sheets are clearly resolved for the first time around the Gamma point. The overall electronic structure shows significant difference from the band structure calculations. Qualitative agreement between the measured and calculated band structure is realized by assuming a chemical potential shift of -0.2 eV. The obvious band renormalization suggests the importance of electron correlation in understanding the electronic structure of the Fe-based compounds.
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We performed an angle-resolved photoemission spectroscopy study of the Ni-based superconductor SrNi$_2$As$_2$. Electron and hole Fermi surface pockets are observed, but their different shapes and sizes lead to very poor nesting conditions. The experimental electronic band structure of SrNi$_2$As$_2$ is in good agreement with first-principles calculations after a slight renormalization (by a factor 1.1), confirming the picture of Hunds exchange-dominated electronic correlations decreasing with increasing filling of the $3d$ shell in the Fe-, Co- and Ni-based compounds. These findings emphasize the importance of Hunds coupling and $3d$-orbital filling as key tuning parameters of electronic correlations in transition metal pnictides.
The (Ca,R)FeAs2 (R=La,Pr and etc.) superconductors with a signature of superconductivity transition above 40 K possess a new kind of block layers that consist of zig-zag As chains. In this paper, we report the electronic structure of the new (Ca,La)FeAs2 superconductor investigated by both band structure calculations and high resolution angle-resolved photoemission spectroscopy measurements. Band structure calculations indicate that there are four hole-like bands around the zone center $Gamma$(0,0) and two electron-like bands near the zone corner M(pi,pi) in CaFeAs2. In our angle-resolved photoemission measurements on (Ca0.9La0.1})FeAs2, we have observed three hole-like bands around the Gamma point and one electron-like Fermi surface near the M(pi,pi) point. These results provide important information to compare and contrast with the electronic structure of other iron-based compounds in understanding the superconductivity mechanism in the iron-based superconductors.
We present a comprehensive study of the low-energy band structure and Fermi surface (FS) topology of $A$Co$_2$As$_2$ ($A=$ Ca, Sr, Ba, Eu) using high-resolution angle-resolved photoemission spectroscopy. The experimental FS topology and band dispersion data are compared with theoretical full-potential linearized augmented-plane-wave (FP-LAPW) calculations, which yielded reasonably good agreement. We demonstrate that the FS maps of $A$Co$_2$As$_2$ are significantly different from those of the parent compounds of Fe-based high-temperature superconductors. Further, the FSs of CaCo$_2$As$_2$ do not show significant changes across its antiferromagnetic transition temperature. The band dispersions extracted in different momentum $(k_{it x}, k_{it y})$ directions show a small electron pocket at the center and a large electron pocket at the corner of the Brillouin zone (BZ). The absence of the hole FS in these compounds does not allow nesting between pockets at the Fermi energy ({it E}$_{rm F}$), which is in contrast to $A$Fe$_2$As$_2$-type parent compounds of the iron-based superconductors. Interestingly, we find that the hole bands are moved 300--400~meV below $E_{rm F}$ depending on the $A$ element. Moreover, the existence of nearly flat bands in the vicinity of $E_{rm F}$ are consistent with the large density of states at $E_{rm F}$. These results are important to understand the physical properties as well as the possibility of the emergence of superconductivity in related materials.
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We introduce a formalism for calculating dynamic response functions using experimental single particle Greens functions derived from angle resolved photoemission spectroscopy (ARPES). As an illustration of this procedure we estimate the dynamic spin response of the cuprate superconductor Bi$_2$Sr$_2$CaCu$_2$O$_{8+delta}$. We find good agreement with superconducting state neutron data, in particular the $(pi,pi)$ resonance with its unusual `reversed magnon dispersion. We anticipate our formalism will also be of useful in interpreting results from other spectroscopies, such as optical and Raman responses.
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