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Register a new userUpper critical field, penetration depth, and depinning frequency of the novel high-temperature superconductor LaFeAsO$_{0.9}$F$_{0.1}$ studied by microwave surface impedance
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Alessandro Narduzzo
Publication date
2008
fields
Physics
and research's language is
English
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Temperature and magnetic field dependent measurements of the microwave surface impedance of superconducting LaFeAsO$_{0.9}$F$_{0.1}$ (Tc $approx$ 26K) reveal a very large upper critical field ($B_{rm c2} approx 56$T) and a large value of the depinning frequency ($f_{0}approx 6$GHz); together with an upper limit for the effective London penetration depth, $lambda_{rm eff} le 200 rm nm$, our results indicate a strong similarity between this system and the high-$T_{rm c}$ superconducting cuprates.
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This paper is no longer active and will NOT appear in print. For new data and analysis, please see: arXiv:0903.2220
The superconducting penetration depth, $lambda(T)$, has been measured in RFeAsO$_{0.9}$F$_{0.1}$ (R=La,Nd) single crystals (R-1111). In Nd-1111, we find an upturn in $lambda(T)$ upon cooling and attribute it to the paramagnetism of the Nd ions, similar to the case of the electron-doped cuprate Nd-Ce-Cu-O. After the correction for paramagnetism, the London penetration depth variation is found to follow a power-law behavior, $Delta lambda_L(T)propto T^{2}$ at low temperatures. The same $T^2$ variation of $lambda(T)$ was found in non-magnetic La-1111 crystals. Analysis of the superfluid density and of penetration depth anisotropy over the full temperature range is consistent with two-gap superconductivity. Based on this and on our previous work, we conclude that both the RFeAsO (1111) and BaFe$_2$As$_2$ (122) families of pnictide superconductors exhibit unconventional two-gap superconductivity.
We will probe the intrinsic behavior of spin susceptibility chi_(spin) in the LaFeAsO(1-x)F(x) superconductor (x ~ 0.1, Tc ~ 27K) using 19-F and 75-As NMR techniques. Our new results firmly establish the pseudo-gap behavior with Delta_(PG)/kB ~ 140K. The estimated magnitude of chi_(spin) at 290K, ~1.8x10^(-4) [emu/mol-Fe], is approximately twice larger than that in high Tc cuprates. We also show that chi_(spin) levels off below ~50K down to Tc.
We show on a few examples of one-band materials with spheroidal Fermi surfaces and anisotropic order parameters that anisotropies $gamma_H$ of the upper critical field and $gamma_lambda$ of the London penetration depth depend on temperature, the feature commonly attributed to multi-band superconductors. The parameters $gamma_H$ and $gamma_lambda$ may have opposite temperature dependencies or may change in the same direction depending on Fermi surface shape and on character of the gap nodes. For two-band systems, the behavior of anisotropies is affected by the ratios of bands densities of states, Fermi velocities, anisotropies, and order parameters. We investigate in detail the conditions determining the directions of temperature dependences of the two anisotropy factors.
Magneto-optical imaging was used to study the local magnetization in polycrystalline NdFeAsO$_{0.9}$F$_{0.1}$ (NFAOF). Individual crystallites up to $sim200times100times30$ $mu m^{3}$ in size could be mapped at various temperatures. The in-grain, persistent current density is about $jsim10^{5}$ A/cm$^{2}$ and the magnetic relaxation rate in a remanent state peaks at about $T_{m}sim38$ K. By comparison with with the total magnetization measured in a bar-shaped, dense, polycrystalline sample, we suggest that NdFeAsO$_{0.9}$F$_{0.1}$ is similar to a layered high-$T_{c}$, compound such as Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+x}$ and exhibits a $3Dto2D$ crossover in the vortex structure. The 2D Ginzburg parameter is about $Gi^{2D}% simeq10^{-2}$ implying electromagnetic anisotropy as large as $epsilon sim1/30$. Below $T_{m}$, the static and dynamic behaviors are consistent with collective pinning and creep.
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