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Register a new userCan antiferromagnetism and superconductivity coexist in the high-field paramagnetic superconductor Nd(O,F)FeAs?
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We present measurements of the temperature and field dependencies of the magnetization M(T,H) of Nd(O0.89F0.11)FeAs at fields up to 33T, which show that superconductivity with the critical temperature Tc ~ 51K cannot coexist with antiferromagnetic ordering. Although M(T,H) at 55 < T < 140K exhibits a clear Curie-Weiss temperature dependence corresponding to the Neel temperature TN ~ 11-12K, the behavior of M(T,H) below Tc is only consistent with either paramagnetism of weakly interacting magnetic moments or a spin glass state. We suggest that the anomalous magnetic behavior of an unusual high-field paramagnetic superconductor Nd(O1-xFx)FeAs is mostly determined by the magnetic Nd ions.
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We report measurements of the phonon density-of-states in iron oxypnictide superconductors by inelastic x-ray scattering. A good agreement with ab-initio calculations that do not take into account strong electronic correlations is found, and an unpredicted softening of phonon branches under F doping of these compounds is observed. Raman scattering experiments lead us to conclude that this softening is not related to zone center phonons, and consequently imply an important softening of the relevant phonon branches at finite momentum transfer Q.
The recently discovered quaternary arsenide oxide superconductor La[O1-xFx]FeAs with the superconducting critical transition temperature (Tc) of 26 K [1], has been quickly expanded to another high-Tc superconducting system beyond copper oxides by the replacement of La with other rare earth elements, such as Sm, Ce, and Pr etc. [2-4], and the Pr[O1-xFx]FeAs has become to be the first non-cuprate superconductor that holding a Tc above 50 K. All these arsenide (including phosphide) superconductors formed in a same tetragonal layered structure with the space group P4/nmm which has an alternant stacked Fe-As layer and RO (R = rare earth metals) layer. Here we report the discovery of another superconductor in this system, the neodymium-arsenide Nd[O1-xFx]FeAs with an resistivity onset Tc of 51.9 K, which is the second non-cuprate compound that superconducts above 50 K.
The newly discovered superconductor La(O,F)FeAs (Tc = 26 K) was investigated using the neutron scattering technique. No spin-density-wave (SDW) order was observed in the normal state nor in the superconducting state, both with and without an applied magnetic field of 9 T, consistent with the proposal that SDW and superconductivity are competing in the laminar materials. While our inelastic measurements offer no constraints on the spin dynamic response from d-wave pairing, an upper limit for the magnetic resonance peak predicted from an extended s-wave pairing mechanism is provided. Our measurements also support the energy scale of the calculated phonon spectrum which is used in electron-phonon coupling theory, and fails to produce the high observed Tc.
We report density functional theory calculations for the parent compound LaOFeAs of the newly discovered 26K Fe-based superconductor LaO$_{1-x}$F$_x$FeAs. We find that the ground state is an ordered antiferromagnet, with staggered moment about 2.3$mu_B$, on the border with the Mott insulating state. We fit the bands crossing the Fermi surface, derived from Fe and As, to a tight-binding Hamiltonian using maximally localized Wannier functions on Fe 3d and As 4p orbitals. The model Hamiltonian accurately describes the Fermi surface obtained via first-principles calculations. Due to the evident proximity of superconductivity to antiferromagnetism and the Mott transition, we suggest that the system may be an analog of the electron doped cuprates, where antiferromagnetism and superconductivity coexist.
We report on the phase diagram of antiferromagnetism (AFM) and superconductivity (SC) in three-layered Ba_2Ca_2Cu_3O_6(F,O)_2 by means of Cu-NMR measurements. It is demonstrated that AFM and SC uniformly coexist in three-layered compounds as well as in four- and five-layered ones. The critical hole density p_c for the long range AFM order is determined as p_c ~ 0.075, which is larger than p_c ~ 0.02 and 0.055 in single- and bi-layered compounds, and smaller than p_c ~ 0.08-0.09 and 0.10-0.11 in four- and five-layered compounds, respectively. This variation of p_c is attributed to the magnetic interlayer coupling which becomes stronger as the stacking number of CuO_2 layers increases; that is, the uniform coexistence of AFM and SC is a universal phenomenon in underdoped regions when a magnetic interlayer coupling is strong enough to stabilize an AFM ordering. In addition, we highlight an unusual pseudogap behavior in three-layered compounds -- the gap behavior in low-energy magnetic excitations collapses in an underdoped region where the ground state is the AFM-SC mixed phase.
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