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Register a new userPrecision measurement of the branching ratio in the 6P3/2 decay of BaII with a single trapped ion
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We present a measurement of the branching ratios from the 6P3/2 state of BaII into all dipoleallowed decay channels (6S1/2, 5D3/2 and 5D5/2). Measurements were performed on single 138Ba+ ions in a linear Paul trap with a frequency-doubled mode-locked Ti:Sapphire laser resonant with the 6S1/2->6P3/2 transition at 455 nm by detection of electron shelving into the dark 5D5/2 state. By driving a pi Rabi rotation with a single femtosecond pulse, a absolute measurement of the branching ratio to 5D5/2 state was performed. Combined with a measurement of the relative decay rates into 5D3/2 and 5D5/2 states performed with long trains of highly attenuated 455 nm pulses, it allowed the extraction of the absolute ratios of the other two decays. Relative strengths normalized to unity are found to be 0.756+/-0.046, 0.0290+/-0.0015 and 0.215+/-0.0064 for 6S1/2, 5D3/2 and 5D5/2 respectively. This approximately constitutes a threefold improvement over the best previous measurements and is a sufficient level of precision to compare to calculated values for dipole matrix elements.
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We present the first terrestrial measurement of the Lande g factor of the 5D5/2 state of singly ionized barium. Measurements were performed on single Doppler-cooled 138Ba+ ions in a linear Paul trap. A frequency-stabilized fiber laser with nominal wavelength 1.762 um was scanned across the 6S1/2<->5D5/2 transition to spectroscopically resolve transitions between Zeeman sublevels of the ground and excited states. From the relative positions of the four narrow transitions observed at several different values for the applied magnetic field, we find a value of 1.2020+/-0.0005 for g of 5D5/2.
Using a single trapped barium ion we have developed an rf spectroscopy technique to measure the ratio of the off-resonant vector ac Stark effect (or light shift) in the 6S_{1/2} and 5D_{3/2} states to 0.1% precision. We find R = Delta_S / Delta_D = -11.494(13) at 514.531 nm where Delta_{S,D} are the light shifts of the m = +/- 1/2 splittings due to circularly polarized light. Comparison of this result with an ab initio calculation of R would yield a new test of atomic theory. By appropriately choosing an off-resonant light shift wavelength one can emphasize the contribution of one or a few dipole matrix elements and precisely determine their values.
We report an improved measurement of the Lande g factor of the 5D5/2 state of singly ionized barium. Measurements were performed on single Doppler-cooled 138Ba+ ions in linear Paul traps using two similar, independent apparatuses. Transitions between Zeeman sublevels of the 6S1/2 and 5D5/2 states were driven with two independent, stabilized radio-frequency synthesizers using a dedicated electrode within each ion trap chamber. State detection within each Zeeman manifold was achieved with a frequency-stabilized fiber laser operating at 1.76 microns. By calculating the ratio of the two Zeeman splittings, and using the measured Lande g factor of the 6S1/2 state, we find a value of 1.200371(4stat)(6sys) for g of 5D5/2.
We demonstrate a new method for the direct measurement of atomic dipole transition matrix elements based on techniques developed for quantum information purposes. The scheme consists of measuring dispersive and absorptive off-resonant light-ion interactions and is applicable to many atomic species. We determine the dipole matrix element pertaining to the Ca II H line, i.e. the 4$^2$S$_{1/2} leftrightarrow $ 4$^2$P$_{1/2}$ transition of $^{40}$Ca$^+$, for which we find the value 2.8928(43) ea$_0$. Moreover, the method allows us to deduce the lifetime of the 4$^2$P$_{1/2}$ state to be 6.904(26) ns, which is in agreement with predictions from recent theoretical calculations and resolves a longstanding discrepancy between calculated values and experimental results.
We define and measure the ratio (R) of the vector ac-Stark effect (or light shift) in the 6S_1/2 and 5D_3/2 states of a single trapped barium ion to 0.2% accuracy at two different off-resonant wavelengths. We earlier found R = -11.494(13) at 514.531nm and now report the value at 1111.68nm, R = +0.4176(8). These observations together yield a value of the <5D||er||4F> matrix element, previously unknown in the literature. Also, comparison of our results with an ab initio calculation of dynamic polarizability would yield a new test of atomic theory and improve the understanding of atomic structure needed to interpret a proposed atomic parity violation experiment.
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