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Quantised Vortices in an Exciton-Polariton Fluid

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 Publication date 2008
  fields Physics
and research's language is English




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One of the most striking quantum effects in a low temperature interacting Bose gas is superfluidity. First observed in liquid 4He, this phenomenon has been intensively studied in a variety of systems for its amazing features such as the persistence of superflows and the quantization of the angular momentum of vortices. The achievement of Bose-Einstein condensation (BEC) in dilute atomic gases provided an exceptional opportunity to observe and study superfluidity in an extremely clean and controlled environment. In the solid state, Bose-Einstein condensation of exciton polaritons has now been reported several times. Polaritons are strongly interacting light-matter quasi-particles, naturally occurring in semiconductor microcavities in the strong coupling regime and constitute a very interesting example of composite bosons. Even though pioneering experiments have recently addressed the propagation of a fluid of coherent polaritons, still no conclusive evidence is yet available of its superfluid nature. In the present Letter, we report the observation of spontaneous formation of pinned quantised vortices in the Bose-condensed phase of a polariton fluid by means of phase and amplitude imaging. Theoretical insight into the possible origin of such vortices is presented in terms of a generalised Gross-Pitaevskii equation. The implications of our observations concerning the superfluid nature of the non-equilibrium polariton fluid are finally discussed.



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Semiconductor microcavity polaritons in the optical parametric scattering regime have been recently demonstrated to display a new variety of dissipationless superfluid behaviour. We report the first observation in resonantly pumped exciton polaritons of a metastable persistent superflow carrying quantum of angular momentum, m. The quantised vortex, excited by a weak 2 ps pulsed probe, is shown to last for at least 80 ps, limited only by the leaking outside the cavity. The polariton circulating superfluid persists in the absence of the driving rotating probe with no apparent dissipation. In addition, for a moving superfluid, we show the coherent splitting of a quantised double vortex, with charge m=2, into two singly quantised vortices of m=1. Remarkably, we observe the m=2 vortex to be stable when they are at rest. The experimental results are compared with a theoretical analysis, obtained describing the triggered parametric scattering regime of polaritons via a two-component Gross-Pitaevskii equation, including pump and decay processes.
We introduce the phenomenon of spiraling vortices in driven-dissipative (non-equilibrium) exciton-polariton condensates excited by a non-resonant pump beam. At suitable low pump intensities, these vortices are shown to spiral along circular trajectories whose diameter is inversely proportional to the effective mass of the polaritons, while the rotation period is mass independent. Both diameter and rotation period are inversely proportional to the pump intensity. Stable spiraling patterns in the form of complexes of multiple mutually-interacting vortices are also found. At elevated pump intensities, which create a stronger homogeneous background, we observe more complex vortex trajectories resembling Spirograph patterns.
Singly quantized vortices have been already observed in many systems including the superfluid helium, Bose Einstein condensates of dilute atomic gases, and condensates of exciton polaritons in the solid state. Two dimensional superfluids carrying spin are expected to demonstrate a different type of elementary excitations referred to as half quantum vortices characterized by a pi rotation of the phase and a pi rotation of the polarization vector when circumventing the vortex core. We detect half quantum vortices in an exciton-polariton condensate by means of polarization resolved interferometry, real space spectroscopy and phase imaging. Half quantum vortices coexist with single quantum vortices in our sample.
Quantum vortices, the quantized version of classical vortices, play a prominent role in superfluid and superconductor phase transitions. However, their exploration at a particle level in open quantum systems has gained considerable attention only recently. Here we study vortex pair interactions in a resonant polariton fluid created in a solid-state microcavity. By tracking the vortices on picosecond time scales, we reveal the role of nonlinearity, as well as of density and phase gradients, in driving their rotational dynamics. Such effects are also responsible for the split of composite spin-vortex molecules into elementary half-vortices, when seeding opposite vorticity between the two spinorial components. Remarkably, we also observe that vortices placed in close proximity experience a pull-push scenario leading to unusual scattering-like events that can be described by a tunable effective potential. Understanding vortex interactions can be useful in quantum hydrodynamics and in the development of vortex-based lattices, gyroscopes, and logic devices.
We demonstrate, both experimentally and theoretically, a new phenomenon: the presence of dissipative coupling in the system of driven bosons. This is evidenced for a particular case of externally excited spots of exciton-polariton condensates in semiconductor microcavities. We observe that for two spatially separated condensates the dissipative coupling leads to the phase locking, either in-phase or out-of-phase, between the condensates. The effect depends on the distance between the condensates. For several excited spots, we observe the appearance of spontaneous vorticity in the system.
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