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A Raman study of the Charge-Density-Wave State in A$_{0.3}$MoO$_3$ (A = K,Rb)

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 Added by Paul van Loosdrecht
 Publication date 2007
  fields Physics
and research's language is English




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We report a comparative Raman spectroscopic study of the quasi-one-dimensional charge-density-wave systems ab (A = K, Rb). The temperature and polarization dependent experiments reveal charge-coupled vibrational Raman features. The strongly temperature-dependent collective amplitudon mode in both materials differ by about 3 cm, thus revealing the role of alkali atom. We discus the observed vibrational features in terms of charge-density-wave ground state accompanied by change in the crystal symmetry. A frequency-kink in some modes seen in bb between T = 80 K and 100 K supports the first-order lock-in transition, unlike rb. The unusually sharp Raman lines(limited by the instrumental response) at very low temperatures and their temperature evolution suggests that the decay of the low energy phonons is strongly influenced by the presence of the temperature dependent charge density wave gap.



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59 - Yuhang Ren , Zhuan Xu , 2003
Low-energy coherent charge-density wave excitations are investigated in blue bronze (K$_{0.3}$MoO$_{3}$) and red bronze (K$_{0.33}$MoO$_{3}$) by femtosecond pump-probe spectroscopy. A linear gapless, acoustic-like dispersion relation is observed for the transverse phasons with a pronounced anisotropy in K$_{0.33}$MoO$_{3}$. The amplitude mode exhibits a weak (optic-like) dispersion relation with a frequency of 1.67 THz at 30 K. Our results show for the first time that the time-resolved optical technique provides momentum resolution of collective excitations in strongly correlated electron systems.Low-energy coherent charge-density wave excitations are investigated in blue bronze (K$_{0.3}$MoO$_{3}$) and red bronze (K$_{0.33}$MoO$_{3}$) by femtosecond pump-probe spectroscopy. A linear gapless, acoustic-like dispersion relation is observed for the transverse phasons with a pronounced anisotropy in K$_{0.33}$MoO$_{3}$. The amplitude mode exhibits a weak (optic-like) dispersion relation with a frequency of 1.67 THz at 30 K. Our results show for the first time that the time-resolved optical technique provides momentum resolution of collective excitations in strongly correlated electron systems.
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184 - B. F. Hu , P. Zheng , R. H. Yuan 2010
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