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Register a new userForced Imbibition - a Tool for Determining Laplace Pressure, Drag Force and Slip Length in Capillary Filling Experiments
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When a very thin capillary is inserted into a liquid, the liquid is sucked into it: this imbibition process is controlled by a balance of capillary and drag forces, which are hard to quantify experimentally, in particularly considering flow on the nanoscale. By computer experiments using a generic coarse-grained model, it is shown that an analysis of imbibition forced by a controllable external pressure quantifies relevant physical parameter such as the Laplace pressure, Darcys permeability, effective pore radius, effective viscosity, dynamic contact angle and slip length of the fluid flowing into the pore. In determining all these parameters independently, the consistency of our analysis of such forced imbibition processes is demonstrated.
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The dynamics of capillary filling in the presence of chemically coated heterogeneous boundaries is investigated, both theoretically and numerically. In particular, by mapping the equations of front motion onto the dynamics of a dissipative driven oscillator, an analytical criterion for front pinning is derived, under the condition of diluteness of the coating spots. The criterion is tested against two dimensional Lattice Boltzmann simulations, and found to provide satisfactory agreement as long as the width of the front interface remains much thinner than the typical heterogeneity scale of the chemical coating.
Imbibition plays a central role in diverse energy, environmental, and industrial processes. In many cases, the medium has multiple parallel strata of different permeabilities; however, how this stratification impacts imbibition is poorly understood. We address this gap in knowledge by directly visualizing forced imbibition in three-dimensional (3D) porous media with two parallel strata. We find that imbibition is spatially heterogeneous: for small capillary number Ca, the wetting fluid preferentially invades the fine stratum, while for Ca above a threshold value, the fluid instead preferentially invades the coarse stratum. This threshold value depends on the medium geometry, the fluid properties, and the presence of residual wetting films in the pore space. These findings are well described by a linear stability analysis that incorporates crossflow between the strata. Thus, our work provides quantitative guidelines for predicting and controlling flow in stratified porous media.
We report forced radial imbibition of water in a porous medium in a Hele-Shaw cell. Washburns law is confirmed in our experiment. Radial imbibition follows scaling dynamics and shows anomalous roughening dynamics when the front invades the porous medium. The roughening dynamics depend on the flow rate of the injected fluid. The growth exponents increase linearly with an increase in the flow rate while the roughness exponents decrease with an increase in the flow rate. Roughening dynamics of radial imbibition is markedly different from one dimensional imbibition with a planar interface window. Such difference caused by geometric change suggests that universality class for the interface growth is not universal.
We show how the capillary filling of microchannels is affected by posts or ridges on the sides of the channels. Ridges perpendicular to the flow direction introduce contact line pinning which slows, or sometimes prevents, filling; whereas ridges parallel to the flow provide extra surface which may enhances filling. Patterning the microchannel surface with square posts has little effect on the ability of a channel to fill for equilibrium contact angle $theta_e lesssim 30^{mathrm{o}}$. For $theta_e gtrsim 60^{mathrm{o}}$, however, even a small number of posts can pin the advancing liquid front.
Imbibition, the displacement of a nonwetting fluid by a wetting fluid, plays a central role in diverse energy, environmental, and industrial processes. While this process is typically studied in homogeneous porous media with uniform permeabilities, in many cases, the media have multiple parallel strata of different permeabilities. How such stratification impacts the fluid dynamics of imbibition, as well as the fluid saturation after the wetting fluid breaks through to the end of a given medium, is poorly understood. We address this gap in knowledge by developing an analytical model of imbibition in a porous medium with two parallel strata, combined with a pore network model that explicitly describes fluid crossflow between the strata. By numerically solving these models, we examine the fluid dynamics and fluid saturation left after breakthrough. We find that the breakthrough saturation of nonwetting fluid is minimized when the imposed capillary number Ca is tuned to a value Ca$^*$ that depends on both the structure of the medium and the viscosity ratio between the two fluids. Our results thus provide quantitative guidelines for predicting and controlling flow in stratified porous media, with implications for water remediation, oil/gas recovery, and applications requiring moisture management in diverse materials.
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