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Register a new userDecoherence of nuclear spins due to direct dipole-dipole interactions probed by resistively detected nuclear magnetic resonance
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We study decoherence of nuclear spins in a GaAs quantum well structure using resistively detected nuclear magnetic resonance. The transverse decoherence time T2 of 75As nuclei is estimated from Rabi-type coherent oscillations as well as by using spin-echo techniques. By analyzing T2 obtained by decoupling techniques, we extract the role of dipole-dipole interactions as sources of decoherence in GaAs. Under the condition that the device is tilted in an external magnetic field, we exhibit enhanced decoherence induced by the change in strength of the direct dipole-dipole interactions between first nearest-neighbor nuclei. The results agree well with simple numerical calculations.
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The drive to improve the sensitivity of nuclear magnetic resonance (NMR) to smaller and smaller sample volumes has led to the development of a variety of techniques distinct from conventional inductive detection. In this chapter, we focus on the technique of force-detected NMR as one of the most successful in yielding sensitivity improvements. We review the rationale for the technique, its basic principles, and give a brief history of its most important results. We then cover in greater detail its application in the first demonstration of three-dimensional (3D) nuclear magnetic resonance imaging (MRI) with nanometer-scale resolution. Next we present recent developments and likely paths for improvement. Finally, the technique and its potential are discussed in the context of competing and complementary technologies.
We report on the demonstration of the resistively detected nuclear magnetic resonance (RDNMR) of a single InSb two-dimensional electron gas (2DEG) at elevated temperatures up to 4 K. The RDNMR signal of 115In in the simplest pseudospin quantum Hall ferromagnet triggered by a large direct current shows a peak-dip line shape, where the nuclear relaxation time T1 at the peak and the dip is different but almost temperature independent. The large Zeeman, cyclotron, and exchange energy scales of the InSb 2DEG contribute to the persistence of the RDNMR signal at high temperatures.
The main obstacle to coherent control of two-level quantum systems is their coupling to an uncontrolled environment. For electron spins in III-V quantum dots, the random environment is mostly given by the nuclear spins in the quantum dot host material; they collectively act on the electron spin through the hyperfine interaction, much like a random magnetic field. Here we show that the same hyperfine interaction can be harnessed such that partial control of the normally uncontrolled environment becomes possible. In particular, we observe that the electron spin resonance frequency remains locked to the frequency of an applied microwave magnetic field, even when the external magnetic field or the excitation frequency are changed. The nuclear field thereby adjusts itself such that the electron spin resonance condition remains satisfied. General theoretical arguments indicate that this spin resonance locking is accompanied by a significant reduction of the randomness in the nuclear field.
We observe nuclear magnetic resonance (NMR) in the fractional quantum Hall regime at Landau level filling factor $ u=2/3$ from simultaneous measurement of longitudinal resistance and photoluminescence (PL). The dynamic nuclear spin polarization is induced by applying a huge electronic current at the spin phase transition point of $ u=2/3$. The NMR spectra obtained from changes in resistance and PL intensity are qualitatively the same; that is, the Knight shift (spin polarized region) and zero-shift (spin unpolarized region) resonances are observed in both. The observed change in PL intensity is interpreted as a consequence of the trion scattering induced by polarized nuclear spins. We conclude that both detection methods probe almost the same local phenomena.
In order to better understand the origin of multiple quantum transitions observed in superparamagnetic nanoparticles, electron magnetic resonance (EMR) studies have been performed on iron oxide nanoparticles assembled inside the anodic alumina membrane. The positions of both the main resonance and forbidden (double-quantum, 2Q) transitions observed at the half-field demonstrate the characteristic angular dependence with the line shifts proportional to 3cos2q-1, where q is the angle between the channel axis and external magnetic field B. This result can be attributed to the interparticle dipole-dipole interactions within elongated aggregates inside the channels. The angular dependence of the 2Q intensity is found to be proportional to sin2qcos2q, that is consistent with the predictions of quantum-mechanical calculations with the account for the mixing of states by non-secular inter-particle dipole-dipole interactions. Good agreement is demonstrated between different kinds of measurements (magnetization curves, line shifts and 2Q intensity), evidencing applicability of the quantum approach to the magnetization dynamics of superparamagnetic objects.
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