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Ultrafast response of surface electromagnetic waves in an aluminum film perforated with subwavelength hole arrays

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 Publication date 2007
  fields Physics
and research's language is English




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The ultrafast dynamics of surface electromagnetic waves photogenerated on aluminum film perforated with subwavelength holes array was studied in the visible spectral range by the technique of transient photomodulation with 100 fs time resolution. We observed a pronounced blueshift of the resonant transmission band that reveals the important role of plasma attenuation in the optical response of nanohole arrays. The blueshift is inconsistent with plasmonic mechanism of extraordinary transmission and points to the crucial role of interference in the formation of transmission bands. The transient photomodulation spectra were successfully modeled within the Boltzmann equation approach for the electron-phonon relaxation dynamics, involving non-equilibrium hot electrons and quasi-equilibrium phonons.



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We study the ultrafast dynamics of surface electromagnetic waves photogenerated on aluminum film perforated with subwavelength holes array by means of transient photomodulation with 100 fs time resolution. We observed a pronounced blueshift of the resonant transmission band that reveals the important role of plasma attenuation in the dynamics and that is inconsistent with plasmon-polariton mechanism of extraordinary transmission. The transient photomodulation spectra were successfully modeled within the Boltzmann equation approach for the electron-phonon relaxation dynamics, involving non-equilibrium hot electrons and quasi-equilibrium phonons.
We present a fully three-dimensional theoretical study of the extraordinary transmission of light through subwavelength hole arrays in optically thick metal films. Good agreement is obtained with experimental data. An analytical minimal model is also developed, which conclusively shows that the enhancement of transmission is due to tunneling through surface plasmons formed on each metal-dielectric interfaces. Different regimes of tunneling (resonant through a surface plasmon molecule, or sequential through two isolated surface plasmons) are found depending on the geometrical parameters defining the system.
Using a time-resolved optically-pumped scanning optical microscopy technique we demonstrate the laser-driven excitation and propagation of spin waves in a 20-nm film of a ferromagnetic metallic alloy Galfenol epitaxially grown on a GaAs substrate. In contrast to previous all-optical studies of spin waves we employ laser-induced thermal changes of magnetocrystalline anisotropy as an excitation mechanism. A tightly focused 70-fs laser pulse excites packets of magnetostatic surface waves with a $e^{-1}$ propagation length of 3.4 $mu$m, which is comparable with that of permalloy. As a result, laser-driven magnetostatic spin waves are clearly detectable at distances up to 10 $mu$m, which promotes epitaxial Galfenol films to the limited family of materials suitable for magnonic devices. A pronounced in-plane magnetocrystalline anisotropy of the Galfenol film offers an additional degree of freedom for manipulating the spin waves parameters. Reorientation of an in-plane external magnetic field relative to the crystallographic axes of the sample tunes the frequency, amplitude and propagation length of the excited waves.
Black phosphorus has recently emerged as a promising material for high performance electronic and optoelectronic device for its high mobility, tunable mid-infrared bandgap and anisotropic electronic properties. Dynamical evolution of photo excited carriers and its induced change of transient electronic properties are critical for materials high field performance, but remains to be explored for black phosphorus. In this work, we perform angle resolved transient reflection spectroscopy to study the dynamical evolution of anisotropic properties of black phosphorus under photo excitation. We find that the anisotropy of reflectivity is enhanced in the pump induced quasi-equilibrium state, suggesting an extraordinary enhancement of the anisotropy in dynamical conductivity in hot carrier dominated regime. These results raise enormous possibilities of creating high field, angle sensitive electronic, optoelectronic and remote sensing devices exploiting the dynamical electronic anisotropic with black phosphorus.
105 - A. Jain , P. Moitra , Th. Koschny 2016
Created surfaces or meta surfaces, composed of appropriately shaped sub-wavelength structures, namely, meta-atoms, control light at wavelength scales. Historically, meta surfaces have used radiating metallic resonators as wavelength inclusions. However, while resonant optical meta surfaces made from metal have been sub-wavelength in the propagation direction, they are too loss for many applications.
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