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Theory of shot noise in single-walled metallic carbon nanotubes weakly coupled to nonmagnetic and ferromagnetic leads

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 Added by Ireneusz Weymann
 Publication date 2007
  fields Physics
and research's language is English




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We present theoretical study of shot noise in single wall metallic carbon nanotubes weakly coupled to either nonmagnetic or ferromagnetic leads. Using the real-time diagrammatic technique, we calculate the current, Fano factor and tunnel magnetoresistance in the sequential tunneling regime. It is shown that the differential conductance displays characteristic four-fold periodicity, indicating single-electron charging. Such a periodicity is also visible in tunnel magnetoresistance of the system as well as in the Fano factor. The present studies elucidate the impact of ferromagnetic (vs. nonmagnetic) contacts on the transport characteristics under consideration.



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We report a measurement on quantum capacitance of individual semiconducting and small band gap SWNTs. The observed quantum capacitance is remarkably smaller than that originating from density of states and it implies a strong electron correlation in SWNTs.
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We present results of wavelength-dependent ultrafast pump-probe experiments on micelle-suspended single-walled carbon nanotubes. The linear absorption and photoluminescence spectra of the samples show a number of chirality-dependent peaks, and consequently, the pump-probe results sensitively depend on the wavelength. In the wavelength range corresponding to the second van Hove singularities (VHSs), we observe sub-picosecond decays, as has been seen in previous pump-probe studies. We ascribe these ultrafast decays to intraband carrier relaxation. On the other hand, in the wavelength range corresponding to the first VHSs, we observe two distinct regimes in ultrafast carrier relaxation: fast (0.3-1.2 ps) and slow (5-20 ps). The slow component, which has not been observed previously, is resonantly enhanced whenever the pump photon energy resonates with an interband absorption peak, and we attribute it to radiative carrier recombination. Finally, the slow component is dependent on the pH of the solution, which suggests an important role played by H$^+$ ions surrounding the nanotubes.
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