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Register a new userAnomalous Paramagnetic Magnetization in Mixed State of CeCoIn$_5$ single crystals
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Magnetization and torque measurements were performed on CeCoIn$_5$ single crystals to study the mixed-state thermodynamics. These measurements allow the determination of both paramagnetic and vortex responses in the mixed-state magnetization. The paramagnetic magnetization is suppressed in the mixed state with the spin susceptibility increasing with increasing magnetic field. The dependence of spin susceptibility on magnetic field is due to the fact that heavy electrons contribute both to superconductivity and paramagnetism and a large Zeeman effect exists in this system. No anomaly in the vortex response was found within the investigated temperature and field range.
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Torque and magnetization measurements in magnetic fields $H$ up to 14 T were performed on CeCoIn$_5$ single crystals. The amplitude of the paramagnetic torque shows an $H^{2.3}$ dependence in the mixed state and an $H^{2}$ dependence in the normal state. In addition, the mixed-state magnetizations for both $Hparallel c$ and $Hparallel ab$ axes show anomalous behavior after the subtraction of the corresponding paramagnetic contributions as linear extrapolations of the normal-state magnetization. These experimental results point towards a nonlinear paramagnetic magnetization in the mixed state of CeCoIn$_5$, which is a result of the fact that both orbital and Pauli limiting effects dominate in the mixed state.
We present core level non-resonant inelastic x-ray scattering (NIXS) data of the heavy fermion compounds CeCoIn$_5$ and CeRhIn$_5$ measured at the Ce $N_{4,5}$-edges. The higher than dipole transitions in NIXS allow determining the orientation of the $Gamma_7$ crystal-field ground-state orbital within the unit cell. The crystal-field parameters of the Ce$M$In$_5$ compounds and related substitution phase diagrams have been investigated in great detail in the past; however, whether the ground-state wavefunction is the $Gamma_7^+$ ($x^2,-,y^2$) or $Gamma_7^-$ ($xy$ orientation) remained undetermined. We show that the $Gamma_7^-$ doublet with lobes along the (110) direction forms the ground state in CeCoIn$_5$ and CeRhIn$_5$. For CeCoIn$_5$, however, we find also some contribution of the first excited state crystal-field state in the ground state due to the stronger hybridization of 4$f$ and conduction electrons, suggesting a smaller $alpha^2$ value than originally anticipated from x-ray absorption. A comparison is made to the results of existing density functional theory plus dynamical mean-field theory calculations.
We investigated the effect of electron and hole doping on the high-field low-temperature superconducting state in CeCoIn$_5$ by measuring specific heat of CeCo(In$_{rm 1-x}$M$_{rm x}$)$_5$ with M=Sn, Cd and Hg and $x$ up to 0.33% at temperatures down to 0.1,K and fields up to 14,T. Although both Cd- and Hg-doping (hole-doping) suppresses the zero-field $T_c$ monotonically, $H_{c2}$ increases with small amounts of doping and has a maximum around $x$=0.2% (M=Cd). On the other hand, with Sn-doping (electron-doping) both zero-field $T_c$ and $H_{c2}$ decrease monotonically. The critical temperature for the high-field low-temperature superconducting state (so called {it Q}-state) correlates with $H_{c2}$ and $T_c$, which we interpret in support of the superconducting origin of this state.
Quantum well states appear in metallic thin films due to the confinement of the wave function by the film interfaces. Using angle-resolved photoemission spectroscopy, we unexpectedly observe quantum well states in fractured single crystals of CeCoIn$_5$. We confirm that confinement occurs by showing that these states binding energies are photon-energy independent and are well described with a phase accumulation model, commonly applied to quantum well states in thin films. This indicates that atomically flat thin films can be formed by fracturing hard single crystals. For the two samples studied, our observations are explained by free-standing flakes with thicknesses of 206 and 101 r{A}. We extend our analysis to extract bulk properties of CeCoIn$_5$. Specifically, we obtain the dispersion of a three-dimensional band near the zone center along in-plane and out-of-plane momenta. We establish part of its Fermi surface, which corresponds to a hole pocket centered at $Gamma$. We also reveal a change of its dispersion with temperature, a signature that may be caused by the Kondo hybridization.
Anomalous paramagnetic effects in dc magnetization were observed in the mixed state of LuNi2B2C, unlike any reported previously. It appears as a kink-like feature for H > 30 kOe and becomes more prominent with increasing field. A specific heat jump at the corresponding temperature suggests that the anomaly is due to a true bulk transition. A magnetic flux transition from a square to an hexagonal lattice is consistent with the anomaly.
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