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Register a new userFemtosecond Photoionization of Atoms under Noise
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We investigate the effect of incoherent perturbations on atomic photoionization due to a femtosecond mid-infrared laser pulse by solving the time-dependent stochastic Schrodinger equation. For a weak laser pulse which causes almost no ionization, an addition of a Gaussian white noise to the pulse leads to a significantly enhanced ionization probability. Tuning the noise level, a stochastic resonance-like curve is observed showing the existence of an optimum noise for a given laser pulse. Besides studying the sensitivity of the obtained enhancement curve on the pulse parameters, such as the pulse duration and peak amplitude, we suggest that experimentally realizable broadband chaotic light can also be used instead of the white noise to observe similar features. The underlying enhancement mechanism is analyzed in the frequency-domain by computing a frequency-resolved atomic gain profile, as well as in the time-domain by controlling the relative delay between the action of the laser pulse and noise.
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We develop a formalism for photoionization (PI) and potential energy curves (PECs) of Rydberg atoms in ponderomotive optical lattices and apply it to examples covering several regimes of the optical-lattice depth. The effect of lattice-induced PI on Rydberg-atom lifetime ranges from noticeable to highly dominant when compared with natural decay. The PI behavior is governed by the generally rapid decrease of the PI cross sections as a function of angular-momentum ($ell$), and by lattice-induced $ell$-mixing across the optical-lattice PECs. In GHz-deep lattices, $ell$-mixing leads to a rich PEC structure, and the significant low-$ell$ PI cross sections are distributed over many lattice-mixed Rydberg states. In lattices less than several tens-of-MHz deep, atoms on low-$ell$ PECs are essentially $ell$-mixing-free and maintain large PI cross sections, while atoms on high-$ell$ PECs trend towards being PI-free. Characterization of PI in GHz-deep Rydberg-atom lattices may be beneficial for optical control and quantum-state manipulation of Rydberg atoms, while data on PI in shallower lattices are potentially useful in high-precision spectroscopy and quantum-computing applications of lattice-confined Rydberg atoms.
We study the robustness of geometric phase in the presence of parametric noise. For that purpose we consider a simple case study, namely a semiclassical particle which moves adiabatically along a closed loop in a static magnetic field acquiring the Dirac phase. Parametric noise comes from the interaction with a classical environment which adds a Brownian component to the path followed by the particle. After defining a gauge invariant Dirac phase, we discuss the first and second moments of the distribution of the Dirac phase angle coming from the noisy trajectory.
Simultaneous quantum estimation of multiple parameters has recently become essential in quantum metrology. Although the ultimate sensitivity of a multiparameter quantum estimation in noiseless environments can beat the standard quantum limit that every classical sensor is bounded by, it is unclear whether the quantum sensor has an advantage over the classical one under realistic noise. In this work, we present a framework of the simultaneous estimation of multiple parameters with quantum sensors in a certain noisy environment. Our multiple parameters to be estimated are three components of an external magnetic field, and we consider the noise that causes only dephasing. We show that there is an optimal sensing time in the noisy environment and the sensitivity can beat the standard quantum limit when the noisy environment is non-Markovian.
Photoionization of a cold atomic sample offers intriguing possibilities to observe collective effects at extremely low temperatures. Irradiation of a rubidium condensate and of cold rubidium atoms within a magneto-optical trap with laser pulses ionizing through 1-photon and 2-photon absorption processes has been performed. Losses and modifications in the density profile of the remaining trapped cold cloud or the remaining condensate sample have been examined as function of the ionizing laser parameters. Ionization cross-sections were measured for atoms in a MOT, while in magnetic traps losses larger than those expected for ionization process were measured.
We measure the photoionization cross-section of vibrationally excited levels in the S2 state of azulene by femtosecond pump-probe spectroscopy. At the wavelengths studied (349-265 nm in the pump) the transient signals exhibit two distinct and well-defined behaviours: (i) Short-term (on the order of a picosecond) polarization dependent transients and (ii) longer (10 ps - 1 ns) time-scale decays. This letter focuses on the short time transient. In contrast to an earlier study by Diau et al.22 [J. Chem. Phys. 110 (1999) 9785.] we unambiguously assign the fast initial decay signal to rotational dephasing of the initial alignment created by the pump transition.
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