Tunnelling of material particles through a classically impenetrable barrier constitutes one of the hallmark effects of quantum physics. When interactions between the particles compete with their mobility through a tunnel junction, intriguing novel dynamical behaviour can arise where particles do not tunnel independently. In single-electron or Bloch transistors, for example, the tunnelling of an electron or Cooper pair can be enabled or suppressed by the presence of a second charge carrier due to Coulomb blockade. Here we report on the first direct and time-resolved observation of correlated tunnelling of two interacting atoms through a barrier in a double well potential. We show that for weak interactions between the atoms and dominating tunnel coupling, individual atoms can tunnel independently, similar to the case in a normal Josephson junction. With strong repulsive interactions present, two atoms located on one side of the barrier cannot separate, but are observed to tunnel together as a pair in a second order co-tunnelling process. By recording both the atom position and phase coherence over time, we fully characterize the tunnelling process for a single atom as well as the correlated dynamics of a pair of atoms for weak and strong interactions. In addition, we identify a conditional tunnelling regime, where a single atom can only tunnel in the presence of a second particle, acting as a single atom switch. Our work constitutes the first direct observation of second order tunnelling events with ultracold atoms, which are the dominating dynamical effect in the strongly interacting regime. Similar second-order processes form the basis of superexchange interactions between atoms on neighbouring lattice sites of a periodic potential, a central component of quantum magnetism.
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