Experimental studies of 152Sm using multiple-step Coulomb excitation and inelastic neutron scattering provide key data that clarify the low-energy collective structure of this nucleus. No candidates for two-phonon beta-vibrational states are found. Experimental level energies of the ground-state and first excited (0+ state) rotational bands, electric monopole transition rates, reduced quadrupole transition rates, and the isomer shift of the first excited 2+ state are all described within ~10% precision using two-band mixing calculations. The basic collective structure of 152Sm is described using strong mixing of near-degenerate coexisting quasi-rotational bands with different deformations.