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Register a new userSemiclassical Dynamics of Electron Wave Packet States with Phase Vortices
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We consider semiclassical higher-order wave packet solutions of the Schrodinger equation with phase vortices. The vortex line is aligned with the propagation direction, and the wave packet carries a well-defined orbital angular momentum (OAM) $hbar l$ ($l$ is the vortex strength) along its main linear momentum. The probability current coils around momentum in such OAM states of electrons. In an electric field, these states evolve like massless particles with spin $l$. The magnetic-monopole Berry curvature appears in momentum space, which results in a spin-orbit-type interaction and a Berry/Magnus transverse force acting on the wave packet. This brings about the OAM Hall effect. In a magnetic field, there is a Zeeman interaction, which, can lead to more complicated dynamics.
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We formulate symmetries in semiclassical Gaussian wave packet dynamics and find the corresponding conserved quantities, particularly the semiclassical angular momentum, via Noethers theorem. We consider two slightly different formulations of Gaussian wave packet dynamics; one is based on earlier works of Heller and Hagedorn, and the other based on the symplectic-geometric approach by Lubich and others. In either case, we reveal the symplectic and Hamiltonian nature of the dynamics and formulate natural symmetry group actions in the setting to derive the corresponding conserved quantities (momentum maps). The semiclassical angular momentum inherits the essential properties of the classical angular momentum as well as naturally corresponds to the quantum picture.
A new method for the study of resonant behavior - using wave-packet dynamics - is presented, based on the powerful window operator technique. The method is illustrated and quantified by application to the astrophysically-important example of low-energy $^{12}$C + $^{12}$C collisions. For this selected, potential model test case, the technique is shown to provide both resonance energies and widths in agreement with alternative methods, such as complex-energy scattering-matrix pole searches and scattering phase-shift analyses. The method has a more general capability to study resonance phenomena across disciplines, that involve particles temporarily trapped by potential pockets.
We investigate theoretically electron dynamics under a VUV attosecond pulse train which has a controlled phase delay with respect to an additional strong infrared laser field. Using the strong field approximation and the fact that the attosecond pulse is short compared to the excited electron dynamics, we arrive at a minimal analytical model for the kinetic energy distribution of the electron as well as the photon absorption probability as a function of the phase delay between the fields. We analyze the dynamics in terms of electron wave packet replicas created by the attosecond pulses. The absorption probability shows strong modulations as a function of the phase delay for VUV photons of energy comparable to the binding energy of the electron, while for higher photon energies the absorption probability does not depend on the delay, in line with the experimental observations for helium and argon, respectively.
Free electron beams that carry high values of orbital angular momentum (OAM) possess large magnetic moments along the propagation direction. This makes them an ideal probe for measuring the electronic and magnetic properties of materials, and for fundamental experiments in magnetism. However, their generation requires the use of complex diffractive elements, which usually take the form of nano-fabricated holograms. Here, we show how the limitations of focused ion beam milling in the fabrication of such holograms can be overcome by using electron beam lithography. We demonstrate experimentally the realization of an electron vortex beam with the largest OAM value that has yet been reported (L = 1000hbar), paving the way for even more demanding demonstrations and applications of electron beam shaping.
Using time-dependent density-matrix renormalization group, we study the time evolution of electronic wave packets in the one-dimensional extended Hubbard model with on-site and nearest neighbor repulsion, U and V, respectively. As expected, the wave packets separate into spin-only and charge-only excitations (spin-charge separation). Charge and spin velocities exhibit non-monotonic dependence on V. For small and intermediate values of V, both velocities increase with V. However, the charge velocity exhibits a stronger dependence than that of the spin, leading to a more pronounced spin-charge separation. Charge fractionalization, on the other hand, is weakly affected by V. The results are explained in terms of Luttinger liquid theory in the weak-coupling limit, and an effective model in the strong-coupling regime.
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