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Register a new userMacroscopic effects in attosecond pulse generation
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We examine how the generation and propagation of high-order harmonics in a partly ionized gas medium affect their strength and synchronization. The temporal properties of the resulting attosecond pulses generated in long gas targets can be significantly influenced by macroscopic effects, in particular by the intensity in the medium and the degree of ionization. Under some conditions, the use of gas targets longer than the absorption length can lead to the generation of self-compressed attosecond pulses. We show this effect experimentally, using long argon-filled gas cells as generating medium.
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Parametric amplification of attosecond coherent pulses around 100 eV at the single-atom level is demonstrated for the first time by using the 3D time-dependent Schr{o}dinger equation in high-harmonic generation processes from excited states of He$^+$. We present the attosecond dynamics of the amplification process far from the ionization threshold and resolve the physics behind it. The amplification of a particular central photon energy requires the seed XUV pulses to be perfectly synchronized in time with the driving laser field for stimulated recombination to the He$^+$ ground state and is only produced in a few specific laser cycles in agreement with the experimental measurements. Our simulations show that the amplified photon energy region can be controlled by varying the peak intensity of the laser field. Our results pave the way to the realization of compact attosecond pulse intense XUV lasers with broad applications.
Attosecond science promises to reveal the most fundamental electronic dynamics occurring in matter and it can develop further by meeting two linked technological goals related to high-order harmonic sources: higher photon flux (permitting to measure low cross-section processes) and improved spectral tunability (allowing selectivity in addressing specific electronic transitions). New developments come through parametric waveform synthesis, which provides control over the shape of high-energy electric field transients, enabling the creation of highly-tunable isolated attosecond pulses via high-harmonic generation. Here we show that central energy, spectral bandwidth/shape and temporal duration of the attosecond pulses can be controlled by shaping the laser pulse waveform via two key parameters: the relative-phase between two halves of the multi-octave spanning optical spectrum, and the overall carrier-envelope phase. These results not only promise to expand the experimental possibilities in attosecond science, but also demonstrate coherent strong-field control of free-electron trajectories using tailored optical waveforms.
Attosecond pulses are fundamental for the investigation of valence and core-electron dynamics on their natural timescale. At present the reproducible generation and characterisation of attosecond waveforms has been demonstrated only through the process of high-order harmonic generation. Several methods for the shaping of attosecond waveforms have been proposed, including metallic filters, multilayer mirrors and manipulation of the driving field. However, none of these approaches allow for the flexible manipulation of the temporal characteristics of the attosecond waveforms, and they suffer from the low conversion efficiency of the high-order harmonic generation process. Free Electron Lasers, on the contrary, deliver femtosecond, extreme ultraviolet and X-ray pulses with energies ranging from tens of $mathrm{mu}$J to a few mJ. Recent experiments have shown that they can generate sub-fs spikes, but with temporal characteristics that change shot-to-shot. Here we show the first demonstration of reproducible generation of high energy ($mathrm{mu}$J level) attosecond waveforms using a seeded Free Electron Laser. We demonstrate amplitude and phase manipulation of the harmonic components of an attosecond pulse train in combination with a novel approach for its temporal reconstruction. The results presented here open the way to perform attosecond time-resolved experiments with Free Electron Lasers.
We demonstrate control over attosecond pulse generation and shaping by numerically optimizing the synthesis of few-cycle to sub-cycle driver waveforms. The optical waveform synthesis takes place in an ultrabroad spectral band covering the ultraviolet-infrared domain. These optimized driver waves are used for ultrashort single and double attosecond pulse production (with tunable separation) revealing the potentials of the light wave synthesizer device demonstrated by Wirth et al. [Science 334, 195 (2011)]. The results are also analyzed with respect to attosecond pulse propagation phenomena.
The generation of the shortest isolated attosecond pulses requires both broad spectral bandwidth and control of the spectral phase. Rapid progress has been made in both aspects, leading to the generation of the world-record-shortest 67 as light pulses in 2012, and broadband attosecond continua covering a wide range of extreme ultraviolet and soft x-ray wavelengths. Such pulses have been successfully applied in photoelectron/photoion spectroscopy and the recently developed attosecond transient absorption spectroscopy to study electron dynamics in matter. In this Review, we discuss the significant recent advancement in the generation, characterization, and application of ultrabroadband isolated attosecond pulses with spectral bandwidth comparable to the central frequency, which can in principle be compressed to a single optical cycle.
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