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Register a new userSpectroscopy of Ultracold, Trapped Cesium Feshbach Molecules
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Added by
Hanns-Christoph Naegerl
Publication date
2007
fields
Physics
and research's language is
English
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We explore the rich internal structure of Cs_2 Feshbach molecules. Pure ultracold molecular samples are prepared in a CO_2-laser trap, and a multitude of weakly bound states is populated by elaborate magnetic-field ramping techniques. Our methods use different Feshbach resonances as input ports and various internal level crossings for controlled state transfer. We populate higher partial-wave states of up to eight units of rotational angular momentum (l-wave states). We investigate the molecular structure by measurements of the magnetic moments for various states. Avoided level crossings between different molecular states are characterized through the changes in magnetic moment and by a Landau-Zener tunneling method. Based on microwave spectroscopy, we present a precise measurement of the magnetic-field dependent binding energy of the weakly bound s-wave state that is responsible for the large background scattering length of Cs. This state is of particular interest because of its quantum-halo character.
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We study collisions in an optically trapped, pure sample of ultracold Cs$_2$ molecules in various internal states. The molecular gas is created by Feshbach association from a near-degenerate atomic gas, with adjustable temperatures in the nanokelvin range. We identify several narrow loss resonances, which point to the coupling to more complex molecular states and may be interpreted as Feshbach resonances in dimer-dimer interactions. Moreover, in some molecular states we observe a surprising temperature dependence in collisional loss. This shows that the situation cannot be understood in terms of the usual simple threshold behavior for inelastic two-body collisions. We interpret this observation as further evidence for a more complex molecular structure beyond the well-understood dimer physics.
We observe magnetically tuned collision resonances for ultracold Cs2 molecules stored in a CO2-laser trap. By magnetically levitating the molecules against gravity, we precisely measure their magnetic moment. We find an avoided level crossing which allows us to transfer the molecules into another state. In the new state, two Feshbach-like collision resonances show up as strong inelastic loss features. We interpret these resonances as being induced by Cs4 bound states near the molecular scattering continuum. The tunability of the interactions between molecules opens up novel applications such as controlled chemical reactions and synthesis of ultracold complex molecules.
Feshbach resonances are the essential tool to control the interaction between atoms in ultracold quantum gases. They have found numerous experimental applications, opening up the way to important breakthroughs. This Review broadly covers the phenomenon of Feshbach resonances in ultracold gases and their main applications. This includes the theoretical background and models for the description of Feshbach resonances, the experimental methods to find and characterize the resonances, a discussion of the main properties of resonances in various atomic species and mixed atomic species systems, and an overview of key experiments with atomic Bose-Einstein condensates, degenerate Fermi gases, and ultracold molecules.
We study the spontaneous dissociation of diatomic molecules produced in cold atomic gases via magnetically tunable Feshbach resonances. We provide a universal formula for the lifetime of these molecules that relates their decay to the scattering length and the loss rate constant for inelastic spin relaxation. Our universal treatment as well as our exact coupled channels calculations for $^{85}$Rb dimers predict a suppression of the decay over several orders of magnitude when the scattering length is increased. Our predictions are in good agreement with recent measurements of the lifetime of $^{85}$Rb$_2$.
We present measurements of the binding energies of $^6$Li p-wave Feshbach molecules formed in combinations of the (F = 1/2, m_F = +1/2), (1), and (F = 1/2, m_F = -1/2), (2), states. The binding energies scale linearly with magnetic field detuning for all three resonances. The relative molecular magnetic moments are found to be $113 pm 7 mu$K/G, $111 pm 6 mu$K/G and $118 pm 8 mu$K/G for the (1)-(1), (1)-(2) and (2)-(2) resonances, respectively, in good agreement with theoretical predictions. Closed channel amplitudes and the size of the p-wave molecules are obtained theoretically from full closed-coupled calculations.
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