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Register a new userTemperature dependence of the impurity-induced resonant state in Zn-doped Bi_2Sr_2CaCu_2O$_{8+delta}$ by Scanning Tunneling Spectroscopy
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We report on the temperature dependence of the impurity-induced resonant state in Zn-doped Bi_2Sr_2CaCu_2O$_{8+delta}$ by scanning tunneling spectroscopy at 30 mK < T < 52 K. It is known that a Zn impurity induces a sharp resonant peak in tunnel spectrum at an energy close to the Fermi level. We observed that the resonant peak survives up to 52 K. The peak broadens with increasing temperature, which is explained by the thermal effect. This result provides information to understand the origin of the resonant peak.
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The {}^{17}O NMR spectra of Bi_2Sr_2CaCu_2O$_{8+delta}$ (Bi-2212) single crystals were measured in the temperature range from 4 K to 200 K and magnetic fields from 3 to 29 T, reported here principally at 8 T. The NMR linewidth of the oxygen in the CuO_{2} plane was found to be magnetically broadened with the temperature dependence of a Curie law where the Curie coefficient decreases with increased doping. This inhomogeneous magnetism is an impurity effect intrinsic to oxygen doping and persists unmodified into the superconducting state.
In conventional superconductors, magnetic impurities form an impurity band due to quantum interference of the impurity bound states, leading to suppression of the superconducting transition temperature. Such quantum interference effects can also be expected in d-wave superconductors. Here, we use scanning tunneling microscopy to investigate the effect of multiple non-magnetic impurities on the local electronic structure of the high-temperature superconductor Bi$_{2}$Sr$_{2}$Ca(Cu$_{1-x}$Zn$_{x}$)$_{2}$O$_{8+delta}$. We find several fingerprints of quantum interference of the impurity bound states including: (i) a two-dimensional modulation of local density-of-states with a period of approximately 5.4 AA along the $a$- and $b$-axes, which is indicative of the d-wave superconducting nature of the cuprates; (ii) abrupt spatial variations of the impurity bound state energy; (iii)an appearance of positive energy states; (iv) a split of the impurity bound state. All of these findings provide important insight into how the impurity band in d-wave superconductors is formed.
The resistance noise in a Bi_2Sr_2CaCu_2O$_{8+delta}$ thin film is found to increase strongly in the underdoped regime. While the increase of the raw resistance noise with decreasing temperature appears to roughly track the previously reported pseudogap temperature for this material, standard noise analysis rather suggests that the additional noise contribution is driven by the proximity of the superconductor-insulator transition.
We study sharp low-energy resonance peaks in the local density of states (LDOS) induced by Zn impurities or possible Cu vacancies in superconducting Bi_2Sr_2CaCu_2O_{8+delta}. The measured structure of these near-zero-bias resonances is quantitatively reproduced by an extended impurity potential without invoking internal impurity states or sophisticated tunneling models. The Zn potential extends at least to the nearest-neighbor Cu sites, and the range of order parameter suppression extends at least 8 AA away from the Zn site. We further show that the local spin susceptibilities near Zn impurities increase rather than decrease with decreasing temperature in the superconducting state due to the sharp increase of LDOS near the Fermi level.
We have developed a material specific theoretical framework for modelling scanning tunneling spectroscopy (STS) of high temperature superconducting materials in the normal as well as the superconducting state. Results for $Bi_2Sr_2CaCu_2O_{8+delta}$ (Bi2212) show clearly that the tunneling process strongly modifies the STS spectrum from the local density of states (LDOS) of the $d_{x^2-y^2}$ orbital of Cu. The dominant tunneling channel to the surface Bi involves the $d_{x^2-y^2}$ orbitals of the four neighbouring Cu atoms. In accord with experimental observations, the computed spectrum displays a remarkable asymmetry between the processes of electron injection and extraction, which arises from contributions of Cu $d_{z^2}$ and other orbitals to the tunneling current.
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