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Register a new userElectron Temperature Evolution in Expanding Ultracold Neutral Plasmas
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We have used the free expansion of ultracold neutral plasmas as a time-resolved probe of electron temperature. A combination of experimental measurements of the ion expansion velocity and numerical simulations characterize the crossover from an elastic-collision regime at low initial Gamma_e, which is dominated by adiabatic cooling of the electrons, to the regime of high Gamma_e in which inelastic processes drastically heat the electrons. We identify the time scales and relative contributions of various processes, and experimentally show the importance of radiative decay and disorder-induced electron heating for the first time in ultracold neutral plasmas.
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Ultracold neutral plasmas, formed by photoionizing laser-cooled atoms near the ionization threshold, have electron temperatures in the 1-1000 kelvin range and ion temperatures from tens of millikelvin to a few kelvin. They represent a new frontier in the study of neutral plasmas, which traditionally deals with much hotter systems, but they also blur the boundaries of plasma, atomic, condensed matter, and low temperature physics. Modelling these plasmas challenges computational techniques and theories of non-equilibrium systems, so the field has attracted great interest from the theoretical and computational physics communities. By varying laser intensities and wavelengths it is possible to accurately set the initial plasma density and energy, and charged-particle-detection and optical diagnostics allow precise measurements for comparison with theoretical predictions. Recent experiments using optical probes demonstrated that ions in the plasma equilibrate in a strongly coupled fluid phase. Strongly coupled plasmas, in which the electrical interaction energy between charged particles exceeds the average kinetic energy, reverse the traditional energy hierarchy underlying basic plasma concepts such as Debye screening and hydrodynamics. Equilibration in this regime is of particular interest because it involves the establishment of spatial correlations between particles, and it connects to the physics of the interiors of gas-giant planets and inertial confinement fusion devices.
Recent experiments with ultracold neutral plasmas show an intrinsic heating effect based on the development of spatial correlations. We investigate whether this effect can be reversed, so that imposing strong spatial correlations could in fact lead to cooling of the ions. We find that cooling is indeed possible. It requires, however, a very precise preparation of the initial state. Quantum mechanical zero-point motion sets a lower limit for ion cooling.
We investigate the strongly correlated ion dynamics and the degree of coupling achievable in the evolution of freely expanding ultracold neutral plasmas. We demonstrate that the ionic Coulomb coupling parameter $Gamma_{rm i}$ increases considerably in later stages of the expansion, reaching the strongly coupled regime despite the well-known initial drop of $Gamma_{rm i}$ to order unity due to disorder-induced heating. Furthermore, we formulate a suitable measure of correlation and show th at $Gamma_{rm i}$ calculated from the ionic temperature and density reflects the degree of order in the system if it is sufficiently close to a quasisteady state. At later times, however, the expansion of the plasma cloud becomes faster than the relaxation of correlations, and the system does not reach thermodynamic equilibrium anymore.
A kinetic approach for the evolution of ultracold neutral plasmas including interionic correlations and the treatment of ionization/excitation and recombination/deexcitation by rate equations is described in detail. To assess the reliability of the approximations inherent in the kinetic model, we have developed a hybrid molecular dynamics method. Comparison of the results reveals that the kinetic model describes the atomic and ionic observables of the ultracold plasma surprisingly well, confirming our earlier findings concerning the role of ion-ion correlations [Phys. Rev. A {bf 68}, 010703]. In addition, the molecular dynamics approach allows one to study the relaxation of the ionic plasma component towards thermodynamical equilibrium.
Three-body recombination, an important collisional process in plasmas, increases dramatically at low electron temperatures, with an accepted scaling of T_e^-9/2. We measure three-body recombination in an ultracold neutral xenon plasma by detecting recombination-created Rydberg atoms using a microwave-ionization technique. With the accepted theory (expected to be applicable for weakly-coupled plasmas) and our measured rates we extract the plasma temperatures, which are in reasonable agreement with previous measurements early in the plasma lifetime. The resulting electron temperatures indicate that the plasma continues to cool to temperatures below 1 K.
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