اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدMagnetoelastic couplings in the deformed Kagom{e} quantum spin lattice of volborthite
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Microscopic spin interactions on a deformed Kagom{e} lattice of volborthite are investigated through magnetoelastic couplings. A negative longitudinal magnetostriction $Delta L<0$ in the $b$ axis is observed, which depends on the magnetization $M$ with a peculiar relation of $Delta L/L propto M^{1.3}$. Based on the exchange striction model, it is argued that the negative magnetostriction originates from a pantograph-like lattice change of the Cu-O-Cu chain in the $b$ axis, and that the peculiar dependence arises from the local spin correlation. This idea is supported by DFT+$U$ calculations simulating the lattice change and a finite-size calculation of the spin correlation, indicating that the recently proposed coupled-trimer model is a plausible one.
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