Realization of strong optomechanical coupling in the single-photon level is crucial to study quantum nonlinear effects and manipulate macroscopic object. Here, we propose an alternative method to towards this goal in a hybrid ensemble-optomechanical system. The sizable membrane-ensemble (ME) coupling mediated by the auxiliary mode of the cavity gives rise to polaritons with lower and higher frequencies. By tuning the ME coupling ($lambda_{rm en}$) approaching the critical coupling value ($lambda_c$), the eigen-energy of the low-frequency polariton gives rise to critical behavior (i.e., quantum phase transition) when the ensemble is within or beyond the low-excitation approximations. Using this critical behavior, the single-photon optomechanical coupling between the cavity and the low-frequency polariton can be greatly enhanced by almost three orders of magnitude with feasible parameters, while the coupling between the high-frequency polariton and the cavity is fully decouped. Our proposal provides a novel way to investigating Kerr effect and blockade in single-photon optomechanical systems.
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