ترغب بنشر مسار تعليمي؟ اضغط هنا

Heating leads to liquid-crystal and crystalline order in a two-temperature active fluid of rods

126   0   0.0 ( 0 )
 نشر من قبل Jayeeta Chattopadhyay
 تاريخ النشر 2021
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

We report phase separation and liquid-crystal ordering induced by scalar activity in a system of Soft Repulsive Spherocylinders (SRS) of aspect ratio $L/D = 5 $. Activity was introduced by increasing the temperature of half of the SRS (labeled textit{`hot}) while maintaining the temperature of the other half constant at a lower value (labeled textit{`cold}). The difference between the two temperatures scaled by the lower temperature provides a measure of the activity. Starting from different equilibrium initial phases, we find that activity leads to segregation of the hot and cold particles. Activity also drives the cold particles through a phase transition to a more ordered state and the hot particles to a state of less order compared to the initial equilibrium state. The cold components of a homogeneous isotropic (I) structure acquire nematic (N) and, at higher activity, crystalline (K) order. Similarly, the cold zone of a nematic initial state undergoes smectic (Sm) and crystal ordering above a critical value of activity while the hot component turns isotropic. We find that the hot particles occupy a larger volume and exert an extra kinetic pressure, confining, compressing and provoking an ordering transition of the cold-particle domains.



قيم البحث

اقرأ أيضاً

230 - Aude Caussarieu 2013
We report experimental and numerical evidences that the dynamics of the director of a liquid crystal driven by an electric field close to the critical point of the Freedericksz Transition(FT) is not described by a Landau-Ginzburg (LG) equation as it is usually done in literature. The reasons are related to the very crude approximations done to obtain this equation, to the finite value of the anchoring energy and to small asymmetries on boundary conditions. We also discuss the difference between the use of LG equation for the statics and the dynamics. These results are useful in all cases where FT is used as an example for other orientational transitions.
We study steady-state properties of a bath of active Brownian particles (ABPs) in two dimensions in the presence of two fixed, permeable (hollow) disklike inclusions, whose interior and exterior regions can exhibit mismatching motility (self-propulsi on) strengths for the ABPs. We show that such a discontinuous motility field strongly affects spatial distribution of ABPs and thus also the effective interaction mediated between the inclusions through the active bath. Such net interactions arise from soft interfacial repulsions between ABPs that sterically interact with and/or pass through permeable membranes assumed to enclose the inclusions. Both regimes of repulsion and attractive (albeit with different mechanisms) are reported and summarized in overall phase diagrams.
We present a detailed study of the heating effects in dielectric measurements carried out on a liquid. Such effects come from the dissipation of the electric power in the liquid and give a contribution to the nonlinear third harmonics susceptibility chi_3 which depends on the frequency and temperature. This study is used to evaluate a possible `spurious contribution to the recently measured nonlinear susceptibility of an archetypical glassforming liquid (Glycerol). Those measurements have been shown to give a direct evaluation of the number of dynamically correlated molecules temperature dependence close to the glass transition temperature T_g~190K (Crauste-Thibierge et al., Phys. Rev. Lett 104,165703(2010)). We show that the heating contribution is totally negligible (i) below 204K at any frequency; (ii) for any temperature at the frequency where the third harmonics response chi_3 is maximum. Besides, this heating contribution does not scale as a function of f/f_{alpha}, with f_{alpha}(T) the relaxation frequency of the liquid. In the high frequency range, when f/f_{alpha} >= 1, we find that the heating contribution is damped because the dipoles cannot follow instantaneously the temperature modulation due to the heating phenomenon. An estimate of the magnitude of this damping is given.
We consider an off-lattice liquid crystal pair potential in strictly two dimensions. The potential is purely repulsive and short-ranged. Nevertheless, by means of a single parameter in the potential, the system is shown to undergo a first-order phase transition. The transition is studied using mean-field density functional theory, and shown to be of the isotropic-to-nematic kind. In addition, the theory predicts a large density gap between the two coexisting phases. The first-order nature of the transition is confirmed using computer simulation and finite-size scaling. Also presented is an analysis of the interface between the coexisting domains, including estimates of the line tension, as well as an investigation of anchoring effects.
Using grand-canonical Monte Carlo simulations, we investigate the phase diagram of hard rods of length $L$ with additional contact (sticky) attractions on square and cubic lattices. The phase diagram shows a competition between gas-liquid and orderin g transitions (which are of demixing type on the square lattice for $L ge 7$ and of nematic type on the cubic lattice for $L ge 5$). On the square lattice, increasing attractions initially lead to a stabilization of the isotropic phase. On the cubic lattice, the nematic transition remains of weak first order upon increasing the attractions. In the vicinity of the gas-liquid transition, the coexistence gap of the nematic transition quickly widens. These features are different from nematic transitions in the continuum.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا