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تسجيل مستخدم جديدA Nonequilibrium Information Entropy Approach to Ternary Fission of Actinides
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Ternary fission of actinides probes the state of the nucleus at scission. Light clusters are produced in space and time very close to the scission point. Within the nonequilibrium statistical operator method, a generalized Gibbs distribution is constructed from the information given by the observed yields of isotopes. Using this relevant statistical operator, yields are calculated taking excited states and continuum correlations into account, in accordance with the virial expansion of the equation of state. Clusters with mass number $A le 10$ are well described using the nonequilibrium generalizations of temperature and chemical potentials. Improving the virial expansion, in-medium effects may become of importance in determining the contribution of weakly bound states and continuum correlations to the intrinsic partition function. Yields of larger clusters, which fail to reach this quasi-equilibrium form of the relevant distribution, are described by nucleation kinetics, and a saddle-to-scission relaxation time of about 7000 fm/c is inferred. Light charged particle emission, described by reaction kinetics and virial expansions, may therefore be regarded as a very important tool to probe the nonequilibrium time evolution of actinide nuclei during fission.
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Nuclear fission of heavy (actinide) nuclei results predominantly in asymmetric mass-splits. Without quantum shells, which can give extra binding energy to these mass-asymmetric shapes, the nuclei would fission symmetrically. The strongest shell effec
ts are in spherical nuclei, so naturally the spherical doubly-magic ${^{132}}$Sn nucleus (${Z=50}$ protons), was expected to play a major role. However, a systematic study of fission has shown that the heavy fragments are distributed around ${Z=52}$ to 56, indicating that ${^{132}}$Sn is not the only driver. Reconciling the strong spherical shell effects at ${Z=50}$ with the different ${Z}$ values of fission fragments observed in nature has been a longstanding puzzle. Here, we show that the final mass asymmetry of the fragments is also determined by the extra stability of octupole (pear-shaped) deformations which have been recently confirmed experimentally around $^{144}$Ba (${Z=56}$), one of very few nuclei with shell-stabilized octupole deformation. Using a modern quantum many-body model of superfluid fission dynamics, we found that heavy fission fragments are produced predominantly with ${52-56}$ protons, associated with significant octupole deformation acquired on the way to fission. These octupole shapes favouring asymmetric fission are induced by deformed shells at ${Z=52}$ and 56. In contrast, spherical magic nuclei are very resistant to octupole deformation, which hinders their production as fission fragments. These findings may explain surprising observations of asymmetric fission of lighter than lead nuclei.
For the first time, we apply the temperature dependent relativistic mean field (TRMF) model to study the ternary fission of heavy nucleus using level density approach. The probability of yields of a particular fragment is obtained by evaluating the c
onvolution integrals which employ the excitation energy and the level density parameter for a given temperature calculated within the TRMF formalism. To illustrate, we have considered the ternary fissions in 252Cf, 242Pu and 236U with fixed third fragment A3 = 48Ca, 20O and 16O respectively. The relative yields are studied for the temperatures T = 1, 2 and 3 MeV. For the comparison, the relative yields are also calculated from the single particle energies of the finite range droplet model (FRDM). In general, the larger phase space for the ternary fragmentation is observed indicating that such fragmentations are most probable ones. For T = 2 and 3 MeV, the Sn + Ni + Ca is the most probable combination for the nucleus 252Cf. However, for the nuclei 242Pu and 236U, the maximum fragmentation yields at T = 2 MeV differ from those at T = 3 MeV. For T = 3 MeV, the closed shell (Z = 8) light mass fragments with its corresponding partners has larger yield values. But, at T = 2 MeV Si/P/S are favorable fragments with the corresponding partners. It is noticed that the symmetric binary fragmentation along with the fixed third fragment for 242Pu and 236U are also favored at T = 1 MeV. The temperature dependence of the nuclear shape and the single particle energies are also discussed.
We developed a three-center phenomenological model,able to explain qualitatively the recently obtained experimental results concerning the quasimolecular stage of a light-particle accompanied fission process. It was derived from the liquid drop model
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