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تسجيل مستخدم جديدComment on Nonlinear electromagnetic response and Higgs-mode excitation in BCS superconductors with impurities
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We comment on the latest paper by M. Silaev [Phys. Rev. B {bf 99}, 224511 (2019)]
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Ultrafast responses of BCS superconductor Nb1-xTixN films in a nonadiabatic excitation regime were investigated by using terahertz (THz) pump-THz probe spectroscopy. After an instantaneous excitation with the monocycle THz pump pulse, a transient osc
illation emerges in the electromagnetic response in the BCS gap energy region. The oscillation frequency coincides with the asymptotic value of the BCS gap energy, indicating the appearance of the theoretically-anticipated collective amplitude mode of the order parameter, namely the Higgs amplitude mode. Our result opens a new pathway to the ultrafast manipulation of the superconducting order parameter by optical means.
When a continuous symmetry of a physical system is spontaneously broken, two types of collective modes typically emerge: the amplitude and phase modes of the order-parameter fluctuation. For superconductors, the amplitude mode is recently referred to
as the Higgs mode as it is a condensed-matter analogue of a Higgs boson in particle physics. Higgs mode is a scalar excitation of the order parameter, distinct from charge or spin fluctuations, and thus does not couple to electromagnetic fields linearly. This is why the Higgs mode in superconductors has evaded experimental observations over a half century after the initial theoretical prediction, except for a charge-density-wave coexisting system. With the advance of nonlinear and time-resolved terahertz spectroscopy techniques, however, it has become possible to study the Higgs mode through the nonlinear light-Higgs coupling. In this review, we overview recent progresses on the study of the Higgs mode in superconductors.
In multiband superconductors, multiple collective modes exist associated with the multiple order parameters. Oscillations of the amplitude and the relative phase of the order parameters are called Higgs and Leggett modes, respectively. Recently, it h
as been suggested that nonmagnetic impurity scattering would enhance nonlinear coupling between the Higgs mode and an electromagnetic wave with a frequency located in the superconducting gap region, while its effect on the Leggett mode is still unresolved. Here, we theoretically investigated the nonlinear optical response of multiband Bardeen-Cooper-Schrieffer-type superconductors in the presence of nonmagnetic impurities with a density matrix approach extending the Mattis-Bardeen model of linear response. We found that the drastic enhancement of nonlinear optical response due to the nonmagnetic impurity scattering occurs only for the Higgs modes and not for the Leggett mode. As a result, both the light-induced dynamics of the superconducting gaps and the resulting third-harmonic generation are dominated by the Higgs modes. We also examined the role of quasiparticle excitations to find that they give the subdominant contribution to the third-harmonic generation.
The study of the electromagnetic response in cuprate superconductors plays a crucial role in the understanding of the essential physics of these materials. Here the doping dependence of the electromagnetic response in cuprate superconductors is studi
ed within the kinetic-energy driven superconducting mechanism. The kernel of the response function is evaluated based on the linear response approximation for a purely transverse vector potential, and can be broken up into its diamagnetic and paramagnetic parts. In particular, this paramagnetic part exactly cancels the corresponding diamagnetic part in the normal-state, and then the Meissner effect is obtained within the entire superconducting phase. Following this kernel of the response function, the electromagnetic response calculation in terms of the specular reflection model qualitatively reproduces many of the striking features observed in the experiments. In particular, the local magnetic-field profile follows an exponential law, while the superfluid density exhibits the nonlinear temperature behavior at the lowest temperatures, followed by the linear temperature dependence extending over the most of the superconducting temperature range. Moreover, the maximal value of the superfluid density occurs at around the critical doping $delta_{rm critical}sim 0.16$, and then decreases in both lower doped and higher doped regimes. The theory also shows that the nonlinear temperature dependence of the superfluid density at the lowest temperatures can be attributed to the nonlocal effects induced by the d-wave gap nodes on the electron Fermi surface.
Disorder - impurities and defects violating an ideal order - is always present in solids. It can result in interesting and sometimes unexpected effects in multiband superconductors. Especially if the superconductivity is unconventional thus having ot
her than the usual s-wave symmetry. This paper uses the examples of iron-based pnictides and chalcogenides to examine how both nonmagnetic and magnetic impurities affect superconducting states with $s_pm$ and $s_{++}$ order parameters. We show that disorder causes the transitions between $s_pm$ and $s_{++}$ states and examine observable effects these transitions can produce.
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