Despite extensive search for about a decade, specular Andreev reflection is only recently realized in bilayer graphene-superconductor interface. However, the evolution from the typical retro type Andreev reflection to the unique specular Andreev reflection in single layer graphene has not yet been observed. We investigate this transition by measuring the differential conductance at the van der Walls interface of single layer graphene and NbSe2 superconductor. We find that the normalized conductance becomes suppressed as we pass through the Dirac cone via tuning the Fermi level and bias energy, which manifests the transition from retro to non-retro type Andreev reflection. The suppression indicates the blockage of Andreev reflection beyond a critical angle of the incident electron with respect to the normal between the single layer graphene and the superconductor junction. The results are compared with a theoretical model of the corresponding setup.
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