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A fundamental requirement in the circuit model of quantum information processing is the realization of fault-tolerant multi-qubit quantum gates with entangling capabilities. A key step towards this end is to achieve control of qubit states through geometric phases at very small spatial scales in an effective and feasible way. A spin-electric coupling present in antiferromagnetic triangular single-molecule magnets (SMMs) allows for manipulation of the spin (qubit) states with a great flexibility. Here, we establish an all-electrical two-qubit geometric phase shift gate acting on the four-fold ground state manifold of a triangular SMM, which represents an effective two-qubit state space. We show that a two-qubit quantum gate with arbitrary entangling power can be achieved through the Berry phase effect, induced by adiabatically varying an external electric field in the plane of the molecule.
The ground state of frustrated (antiferromagnetic) triangular molecular magnets is characterized by two total-spin $S =1/2$ doublets with opposite chirality. According to a group theory analysis [M. Trif textit{et al.}, Phys. Rev. Lett. textbf{101},
Using X-band pulsed electron spin resonance, we report the intrinsic spin-lattice ($T_1$) and phase coherence ($T_2$) relaxation times in molecular nanomagnets for the first time. In Cr$_7M$ heterometallic wheels, with $M$ = Ni and Mn, phase coherenc
Coherent control of individual molecular spins in nano-devices is a pivotal prerequisite for fulfilling the potential promised by molecular spintronics. By applying electric field pulses during time-resolved electron spin resonance measurements, we m
Heavy metals are key to spintronics because of their high spin-orbit coupling (SOC) leading to efficient spin conversion and strong magnetic interactions. When C60 is deposited on Pt, the molecular interface is metallised and the spin Hall angle in Y
We discuss Floquet engineering of dissipative molecular systems through periodic driving of an infrared-active vibrational transition, either directly or via a cavity mode. Following a polaron quantum Langevin equations approach, we derive correlatio