We demonstrate several building blocks for an ion-photon interface based on a trapped Ca ion in an optical cavity. We identify a favorable experimental configuration and measure system parameters, including relative motion of the trapped ion and the resonator mode. A complete spectrum of cavity-assisted Raman transitions between the $4^{2}S_{1/2}$ and $3^{2}D_{5/2}$ manifolds is obtained. On two of these transitions, we generate orthogonally polarized cavity photons, and we demonstrate coherent manipulation of the corresponding pair of atomic states. Possible implementations of atom-photon entanglement and state mapping within the ion-cavity system are discussed.
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