The theoretical calculation for nonlinear refractive index in Cr: ZnSe - active medium predicts the strong defocusing cascaded second-order nonlinearity within 2000 - 3000 nm spectral range. On the basis of this result the optimal cavity configuration for Kerr-lens mode locking is proposed that allows to achieve a sub-100 fs pulse duration. The numerical simulations testify about strong destabilizing processes in the laser resulting from a strong self-phase modulation. The stabilization of the ultrashort pulse generation is possible due to spectral filtering that increases the pulse duration up to 300 fs.
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