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A method, based on the Neel-Brown model of thermally activated magnetization reversal of a magnetic single-domain particle, is proposed to study the field sweep rate dependence of the coercive field of single-molecule magnets (SMMs). The application to Mn12 and Mn84 SMMs allows the determination of the important parameters that characterize the magnetic properties: the energy barrier, the magnetic anisotropy constant, the spin, tau_0, and the crossover temperature from the classical to the quantum regime. The method may be particularly valuable for large SMMs that do not show quantum tunneling steps in the hysteresis loops.
In this work we study theoretically the coupling of single molecule magnets (SMMs) to a variety of quantum circuits, including microwave resonators with and without constrictions and flux qubits. The main results of this study is that it is possible
We present studies on magnetic nano-structures with 3D architectures, fabricated using electrodeposition in the pores of well-ordered templates prepared by self-assembly of polystyrene latex spheres. The coercive field is found to demonstrate an osci
We show that the nuclear spin dynamics in the single-molecule magnet Mn12-ac below 1 K is governed by quantum tunneling fluctuations of the cluster spins, combined with intercluster nuclear spin diffusion. We also obtain the first experimental proof
A Mn4 single-molecule magnet (SMM) is used to show that quantum tunneling of magnetization (QTM) is not suppressed by moderate three dimensional exchange coupling between molecules. Instead, it leads to an exchange bias of the quantum resonances whic
Magnetization measurements of a molecular clusters Mn12 with a spin ground state of S = 10 show resonance tunneling at avoided energy level crossings. The observed oscillations of the tunnel probability as a function of the magnetic field applied alo