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We study the nonlinear optical response in a superconducting NbN thin film with strong terahertz (THz)wave. Besides the expected third harmonic generation, we observe a new transient oscillation which softensin frequency with temperature increasing towards superconducting transition temperatureTc. We identify thisnew mode as the Higgs transient oscillation. To verify this proposal, we introduce a time-frequency resolvedtechnique, named spectrogram for visualizing THz spectrum. The dynamic decaying behavior of the mode isobserved, which is consistent with theoretical expectation about intrinsic Higgs oscillation. Moreover, a higherorder nonlinear optics effect,i.e.fifth harmonic generation, has been observed for the first time, which we assignto the higher order coupling between Higgs mode and electromagn
Despite being usually considered two competing phenomena, charge-density-wave and superconductivity coexist in few systems, the most emblematic one being the transition metal dichalcogenide 2H-NbSe$_2$. This unusual condition is responsible for speci
The quest for new functionalities in quantum materials has recently been extended to non-equilibrium states, which are interesting both because they exhibit new physical phenomena and because of their potential for high-speed device applications. Not
When a continuous symmetry of a physical system is spontaneously broken, two types of collective modes typically emerge: the amplitude and phase modes of the order-parameter fluctuation. For superconductors, the amplitude mode is recently referred to
The competing orders in the particle-particle (P-P) channel and the particle-hole (P-H) channel have been proposed separately to explain the pseudogap physics in cuprates. By solving the Bogoliubov-deGennes equation self-consistently, we show that th
The pressure evolution of the Raman active electronic excitations of the transition metal dichalcogenides 2H-TaS$_2$ is followed through the pressure phase diagram embedding incommensurate charge-density-wave and superconducting states. At high press