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Quest for new states of matter near an ordered phase is a promising route for making modern physics forward. By probing thermal properties of a ferroelectric (FE) crystal Ba1-xSrxAl2O4, we have clarified that low-energy excitation of acoustic phonons is remarkably enhanced with critical behavior at the border of the FE phase. The phonon spectrum is significantly damped toward the FE phase boundary and transforms into glasslike phonon excitation which is reminiscent of a boson peak. This system thus links long-standing issues of amorphous solids and structural instability in crystals to pave the way to controlling lattice fluctuation as a new tuning parameter.
To gain control over magnetic order on ultrafast time scales, a fundamental understanding of the way electron spins interact with the surrounding crystal lattice is required. However, measurement and analysis even of basic collective processes such a
Ion diffusion is important in a variety of applications, yet fundamental understanding of the diffusive process in solids is still missing, especially considering the interaction of lattice vibrations (phonons) and the mobile species. In this work, w
We report phonon renormalization induced by an external electric field E in ferroelectric poly(vinylidene fluoride-trifluoroethylene) [P(VDF-TrFE)] nanofibers through measuring the E-dependent thermal conductivity. Our experimental results are in exc
Local inhomogeneities known as polar nanoregions (PNR) play a key role in governing the dielectric properties of relaxor ferroelectrics - a special class of material that exhibits an enormous electromechanical response and is easily polarized with an
Modulating the polarization of a beam of quantum particles is a powerful method to tailor the macroscopic properties of the ensuing energy flux as it directly influences the way in which its quantum constituents interact with other particles, waves o