Dy$_{2}$Zr$_{2}$O$_{7}$ a disordered pyrochlore system, exhibits the spin ice freezing under the application of magnetic field. Our studies suggest the stabilization of pyrochlore phase in Dy$_{2-x}$La$_{x}$Zr$_{2}$O$_{7}$ with the substitution of nonmagnetic La, along with the biphasic mixture for the intermediate compositions. We observed that the higher La compositions (1.5 $leq$ x $leq$ 1.9), show spin freezing (T $sim$ 17 K) similar to the field induced spin ice freezing for low La compositions (0 $leq$ x $leq$ 0.5), and the well known spin ice systems Dy$_{2}$Ti$_{2}$O$_{7}$ and Ho$_{2}$Ti$_{2}$O$_{7}$. The low temperature magnetic state for higher La compositions (1.5 $leq$ x $leq$ 1.9) culminates into spin glass state below 6 K. The Cole-Cole plot and Casimir-du Pr$acute{e}$ fit shows narrow distribution of spin relaxation time in these compounds.
تحميل البحث