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Single-cycle optical pulses with a controlled electromagnetic waveform allow to steer the motion of low-energy electrons in atoms, molecules, nanostructures or condensed-matter on attosecond dimensions in time. However, high-energy electrons under single-cycle light control would be an enabling technology for beam-based attosecond physics with free-electron lasers or electron microscopy. Here we report the control of freely propagating keV electrons with an isolated optical cycle of mid-infrared light and create a modulated electron current with a peak-cycle-specific sub-femtosecond structure in time. The evident effects of the carrier-envelope phase, amplitude and dispersion of the optical waveform on the temporal composition, pulse durations and chirp of the free-space electron wavefunction demonstrate the sub-cycle nature of our control. These results create novel opportunities in laser-driven particle acceleration, seeded free-electron lasers, attosecond space-time imaging, electron quantum optics and wherever else high-energy electrons are needed with the temporal structure of single-cycle light.
Free-electron beams serve as uniquely versatile probes of microscopic structure and composition, and have repeatedly revolutionized atomic-scale imaging, from solid-state physics to structural biology. Over the past decade, the manipulation and inter
In situ generation of a high-energy, high-current, spin-polarized electron beam is an outstanding scientific challenge to the development of plasma-based accelerators for high-energy colliders. In this Letter we show how such a spin-polarized relativ
Compact laser-driven accelerators are versatile and powerful tools of unarguable relevance on societal grounds for the diverse purposes of science, health, security, and technology because they bring enormous practicality to state-of-the-art achievem
The measurement of transient optical fields has proven critical to understanding the dynamical mechanisms underlying ultrafast physical and chemical phenomena, and is key to realizing higher speeds in electronics and telecommunications. Complete char
We theoretically show that a single free electron in circular/spiral motion radiates an electromagnetic wave possessing helical phase structure and carrying orbital angular momentum. We experimentally demonstrate it by double-slit diffraction on radi