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Kondo physics of magnetic adatoms on metallic surfaces when the onset of the surface conduction density of states crosses the Fermi level

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 نشر من قبل Pablo Roura-Bas Dr.
 تاريخ النشر 2019
  مجال البحث فيزياء
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We study the role of the onset of Shockley states, $D_s$, belonging to (111) surfaces of Cu, Ag and Au in the Kondo effect when a magnetic impurity is deposited on them. When $D_s$ approaches to the Fermi level, $E_F$, thing that can be done by compressing (stretching) the metallic sample, we found that most of the thermodynamic and dynamic properties of the impurity are affected in a non trivial way. We model the system by a generic Anderson impurity model and solve it by using the numerical renormalization group, NRG, technique. In particular, the impurity contribution to magnetic susceptibility and entropy as a function of temperature exhibit negative values and goes to zero slowly in a logarithmic shape. Furthermore, we found a suppression of the spectral density weight at the Fermi level when $D_ssim E_F$ even in the Kondo regime. As a consequence, the conductance through the impurity is strongly reduced by near $25%$ of the unitary value $2e^2/h$. Finally, we analyze these features in realistic systems like Co on Ag(111) reported in the literature.



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