ترغب بنشر مسار تعليمي؟ اضغط هنا

Johari-Goldstein relaxation in glass-electrets

130   0   0.0 ( 0 )
 نشر من قبل Peter Lunkenheimer
 تاريخ النشر 2019
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

We investigate the dielectric response in the glass-electret state of two dipolar glass-forming materials. This unusual polar glassy state of matter is produced when a dipolar liquid is supercooled under the influence of a high electric dc field, which leads to partial orientational order of the molecules carrying a dipole moment. Investigation of the prepared glass-electrets by using low-field dielectric spectroscopy reveals a clear modification of their dielectric response in the regime of the Johari-Goldstein beta-relaxation, pointing to a small but significant increase of its relaxation strength compared to the normal glass. We discuss the implications of this finding for the still controversial microscopic interpretation of the Johari-Goldstein relaxation, an inherent property of glassy matter.



قيم البحث

اقرأ أيضاً

We presented that the relaxation of n coupling molecules in a molecular string exhibits n individual relaxation modes (RMs), each mode being characterized by a definite relaxation time and amplitude according to the string model. The n RMs behaving a single relaxation at high temperature, evolves to two relaxation species, at low temperature, with different temperature dependences for the respective relaxation times and amplitudes. Since the characteristics of the two relaxation species are in agreement with those exhibited by the universal alpha- and Johari-Goldstein (JG) beta-relaxations in glass dynamics, we provided a unified molecular level mechanism for these two processes.
The relaxation of the specific heat and the entropy to their equilibrium values is investigated numerically for the three-dimensional Coulomb glass at very low temperatures. The long time relaxation follows a stretched exponential function, $f(t)=f_0 exp[-(t/tau)^beta]$, with the exponent $beta$ increasing with the temperature. The relaxation time follows an Arrhenius behavior divergence when $Tto 0$. A relation between the specific heat and the entropy in the long time regime is found.
64 - L. Saviot , E. Duval , J. F. Jal 2000
Low-frequency Raman and inelastic neutron scattering of amorphous bis-phenol A polycarbonate is measured at low temperature, and compared. The vibrational density of states and light-vibration coupling coefficient are determined. The frequency depend ences of these parameters are explained by propagating vibration modes up to an energy of about 1 meV, and fracton-like modes in more cohesive domains at higher energies. The vibrational dynamics is in agreement with a disorder in the glass, which is principally of bonding or of elasticity instead of density.
115 - Lei-Han Tang 2009
The gauge glass model offers an interesting example of a randomly frustrated system with a continuous O(2) symmetry. In two dimensions, the existence of a glass phase at low temperatures has long been disputed among numerical studies. To resolve this controversy, we examine the behavior of vortices whose movement generates phase slips that destroy phase rigidity at large distances. Detailed analytical and numerical studies of the corresponding Coulomb gas problem in a random potential establish that the ground state, with a finite density of vortices, is polarizable with a scale-dependent dielectric susceptibility. Screening by vortex/antivortex pairs of arbitrarily large size is present to eliminate the logarithmic divergence of the Coulomb energy of a single vortex. The observed power-law decay of the Coulomb interaction between vortices with distance in the ground state leads to a power-law divergence of the glass correlation length with temperature $T$. It is argued that free vortices possess a bound excitation energy and a nonzero diffusion constant at any $T>0$.
123 - J. Bergli , Y. M. Galperin 2012
Slow relaxation and aging of the conductance are experimental features of a range of materials, which are collectively known as electron glasses. We report dynamic Monte Carlo simulations of the standard electron glass lattice model. In a non-equilib rium state, the electrons will often form a Fermi distribution with an effective electron temperature higher than the phonon bath temperature. We study the effective temperature as a function of time in three different situations: relaxation after a quench from an initial random state, during driving by an external electric field and during relaxation after such driving. We observe logarithmic relaxation of the effective temperature after a quench from a random initial state as well as after driving the system for some time $t_w$ with a strong electric field. For not too strong electric field and not too long $t_w$ we observe that data for the effective temperature at different waiting times collapse when plotted as functions of $t/t_w$ -- the so-called simple aging. During the driving period we study how the effective temperature is established, separating the contributions from the sites involved in jumps from those that were not involved. It is found that the heating mainly affects the sites involved in jumps, but at strong driving, also the remaining sites are heated.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا