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Second and third harmonic generation in the opaque region of a GaAs wafer is experimentally observed both in transmission and reflection. These harmonic components can propagate through an opaque material as long as the pump is tuned to a region of transparency or semi-transparency, and correspond to the inhomogeneous solutions of Maxwells equations with nonlinear polarization sources. We show that measurement of the angular and polarization dependence of the observed harmonic components allows one to infer the different nonlinear mechanisms that trigger these processes, including bulk nonlinearity, magnetic Lorentz and surface contributions. Experimental results are compared with a detailed numerical model that takes into account these different effects.
We present a new theoretical approach to the study of second and third harmonic generation from metallic nanostructures and nanocavities filled with a nonlinear material, in the ultrashort pulse regime. We model the metal as a two-component medium, u
We study second harmonic generation in nonlinear, GaAs gratings. We find large enhancement of conversion efficiency when the pump field excites the guided mode resonances of the grating. Under these circumstances the spectrum near the pump wavelength
Nonlinear frequency conversion plays a crucial role in advancing the functionality of next-generation optical systems. Portable metrology references and quantum networks will demand highly efficient second-order nonlinear devices, and the intense non
Tunable coherent light sources operating in the vacuum ultraviolet (VUV) region in 100-200-nm (6-12 eV) wavelength range have important spectroscopic applications in many research fields, including time-resolved angle-resolved photoemission spectrosc
We show a new path to {epsilon}~0 materials without resorting to metal-based metamaterial composites. A medium that can be modeled using Lorentz oscillators usually displays {epsilon}=0 crossing points, e.g. {epsilon}=0 at {lambda}~7{mu}m and 20{mu}m