اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدDual topology in Jacutingaite Pt$_2$HgSe$_3$
78
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
Topological phases of electronic systems often coexist in a material, well-known examples being systems which are both strong and weak topological insulators. More recently, a number of materials have been found to have the topological structure of both a weak topological insulator and a mirror-protected topological crystalline insulator. In this work, we first focus on the naturally occurring mineral called Jacutingaite, Pt$_2$HgSe$_3$, and show based on density-functional calculations that it realizes this dual topological phase and that the same conclusion holds for Pd$_2$HgSe$_3$. Second, we introduce tight-binding models that capture the essential topological properties of this dual topological phase in materials with three-fold rotation symmetry and use these models to describe the main features of the surface spectral density of different materials in the class.
قيم البحث
اقرأ أيضاً
Recently, the very first large-gap Kane-Mele quantum spin Hall insulator was predicted to be monolayer jacutingaite (Pt$_2$HgSe$_3$), a naturally-occurring exfoliable mineral discovered in Brazil in 2008. The stacking of quantum spin Hall monolayers
into a van-der-Waals layered crystal typically leads to a (0;001) weak topological phase, which does not protect the existence of surface states on the (001) surface. Unexpectedly, recent angle-resolved photoemission spectroscopy experiments revealed the presence of surface states dispersing over large areas of the 001-surface Brillouin zone of jacutingaite single crystals. The 001-surface states have been shown to be topologically protected by a mirror Chern number $C_M=-2$, associated with a nodal line gapped by spin-orbit interactions. Here, we extend the two-dimensional Kane-Mele model to bulk jacutingaite and unveil the microscopic origin of the gapped nodal line and the emerging crystalline topological order. By using maximally-localized Wannier functions, we identify a large non-trivial second nearest-layer hopping term that breaks the standard paradigm of weak topological insulators. Complemented by this term, the predictions of the Kane-Mele model are in remarkable agreement with recent experiments and first-principles simulations, providing an appealing conceptual framework also relevant for other layered materials made of stacked honeycomb lattices.
Saddle-point van Hove singularities in the topological surface states are interesting because they can provide a new pathway for accessing exotic correlated phenomena in topological materials. Here, based on first-principles calculations combined wit
h a $mathbf {k cdot p}$ model Hamiltonian analysis, we show that the layered platinum mineral jacutingaite (Pt$_2$HgSe$_3$) harbours saddle-like topological surface states with associated van Hove singularities. Pt$_2$HgSe$_3$ is shown to host two distinct types of nodal lines without spin-orbit coupling (SOC) which are protected by combined inversion ($I$) and time-reversal ($T$) symmetries. Switching on the SOC gaps out the nodal lines and drives the system into a topological insulator state with nonzero weak topological invariant $Z_2=(0;001)$ and mirror Chern number $n_M=2$. Surface states on the naturally cleaved (001) surface are found to be nontrivial with a unique saddle-like energy dispersion with type II van Hove singularities. We also discuss how modulating the crystal structure can drive Pt$_2$HgSe$_3$ into a Dirac semimetal state with a pair of Dirac points. Our results indicate that Pt$_2$HgSe$_3$ is an ideal candidate material for exploring the properties of topological insulators with saddle-like surface states.
Magnetic skyrmions have been the focus of intense research due to their unique qualities which result from their topological protections. Previous work on Cu$_2$OSeO$_3$, the only known insulating multiferroic skyrmion material, has shown that chemic
al substitution alters the skyrmion phase. We chemically substitute Zn, Ag, and S into powdered Cu$_2$OSeO$_3$ to study the effect on the magnetic phase diagram. In both the Ag and the S substitutions, we find that the skyrmion phase is stabilized over a larger temperature range, as determined via magnetometry and small-angle neutron scattering (SANS). Meanwhile, while previous magnetometry characterization suggests two high temperature skyrmion phases in the Zn-substituted sample, SANS reveals the high temperature phase to be skyrmionic while we are unable to distinguish the other from helical order. Overall, chemical substitution weakens helical and skyrmion order as inferred from neutron scattering of the $|$q$| approx$ 0.01 $r{A}^{-1}$ magnetic peak.
Single crystals of a honeycomb lattice antiferromagnet, Tb$_2$Ir$_3$Ga$_9$ were synthesized, and the physical properties have been studied. From magnetometry, a long-range antiferromagnetic ordering at $approx$12.5 K with highly anisotropic magnetic
behavior was found. Neutron powder diffraction confirms that the Tb spins lie along the $va $-axis, parallel to the shortest Tb-Tb contact. Two field-induced spin-flip transitions are observed when the field is applied parallel to this axis, separated by a plateau corresponding roughly to M$approx$M$_{rm{s}}$/2. Transport measurements show the resistivity to be metallic with a discontinuity at the onset of Neel order. Heat capacity shows a $lambda$-like transition confirming the bulk nature of the magnetism. We propose a phenomenological spin-Hamiltonian that describes the magnetization plateau as a result of strong Ising character arising from a quasidoublet ground state of the Tb$^{3+}$ ion in a site of textit{C$_s$} symmetry and expressing a significant bond dependent anisotropy.
We study the fate of the surface states of Bi$_2$Se$_3$ under disorder with strength larger than the bulk gap, caused by neon sputtering and nonmagnetic adsorbates. We find that neon sputtering introduces strong but dilute defects, which can be model
ed by a unitary impurity distribution, whereas adsorbates, such as water vapor or carbon monoxide, are best described by Gaussian disorder. Remarkably, these two disorder types have a dramatically different effect on the surface states. Our soft x-ray ARPES measurements combined with numerical simulations show that unitary surface disorder pushes the Dirac state to inward quintuplet layers, burying it below an insulating surface layer. As a consequence, the surface spectral function becomes weaker, but retains its quasiparticle peak. This is in contrast to Gaussian disorder, which smears out the quasiparticle peak completely. At the surface of Bi$_2$Se$_3$, the effects of Gaussian disorder can be reduced by removing surface adsorbates using neon sputtering, which, however, introduces unitary scatterers. Since unitary disorder has a weaker effect than Gaussian disorder, the ARPES signal of the Dirac surface state becomes sharper upon sputtering.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
