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Strong field driven electric currents in condensed matter systems open new frontiers in petahertz electronics. In this regime new challenges arise as the role of the band structure and the quantum nature of electron-hole dynamics have yet to be resolved. Here we reveal the underlying attosecond dynamics that dictates the temporal evolution of carriers in multi-band solid state systems, via high harmonic generation (HHG) spectroscopy. We demonstrate that when the electron-hole relative velocity approaches zero, enhanced quantum interference leads to the appearance of spectral caustics in the HHG spectrum. Introducing the role of the dynamical joint density of states (JDOS) we identify its direct mapping into the spectrum, exhibiting singularities at the spectral caustics. By probing these singularities, we visualize the structure of multiple unpopulated high conduction bands. Our results open a new path in the control and study of attosecond quasi-particle interactions within the field dressed band structure of crystals.
With its direct correspondence to electronic structure, angle-resolved photoemission spectroscopy (ARPES) is a ubiquitous tool for the study of solids. When extended to the temporal domain, time-resolved (TR)-ARPES offers the potential to move beyond
We present an experimental technique using orbital angular momentum (OAM) in a fundamental laser field to drive High Harmonic Generation (HHG). The mixing of beams with different OAM allows to generate two laser foci tightly spaced to study the phase
High-harmonic generation by a highly non-linear interaction of infrared laser fields with matter allows for the generation of attosecond pulses in the XUV spectral regime. This process, well established for atoms, has been recently extended to the co
We present a numerical study of the resonant high harmonic generation by tin ions in an elliptically-polarised laser field along with a simple analytical model revealing the mechanism and main features of this process. We show that the yield of the r
High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to important applica