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The free-free opacity in dense systems is a property that both tests our fundamental understanding of correlated many-body systems, and is needed to understand the radiative properties of high energy-density plasmas. Despite its importance, predictive calculations of the free-free opacity remain challenging even in the condensed matter phase for simple metals. Here we show how the free-free opacity can be modelled at finite-temperatures via time-dependent density functional theory, and illustrate the importance of including local field corrections, core polarization and self-energy corrections. Our calculations for ground-state Al are shown to agree well with experimental opacity measurements performed on the Artemis laser facility across a wide range of x-ray to ultraviolet wavelengths. We extend our calculations across the melt to the warm-dense matter regime, and find good agreement with advanced plasma models based on inverse bremsstrahlung at temperatures above 10 eV.
We describe a simple method to determine, from ab initio calculations, the complete orientation-dependence of interfacial free energies in solid-state crystalline systems. We illustrate the method with an application to precipitates in the Al-Ti allo
Warm dense matter (WDM) -- an exotic state of highly compressed matter -- has attracted high interest in recent years in astrophysics and for dense laboratory systems. At the same time, this state is extremely difficult to treat theoretically. This i
We calculate the leading corrections to jet momentum broadening and medium-induced branching that arise from the velocity of the moving medium at first order in opacity. These results advance our knowledge of jet quenching and demonstrate how it coup
Last few years have witnessed significant enhancement of thermoelectric figure of merit of lead telluride (PbTe) via nanostructuring. Despite the experimental progress, current understanding of the electron transport in PbTe is based on either band s
We have investigated the ultracold interspecies scattering properties of metastable triplet He and Rb. We performed state-of-the-art ab initio calculations of the relevant interaction potential, and measured the interspecies elastic cross section for