Quantum memories with high efficiency and fidelity are essential for long-distance quantum communication and information processing. Techniques have been developed for quantum memories based on atomic ensembles. The atomic memories relying on the atom-light resonant interaction usually suffer from the limitations of narrow bandwidth. The far-off-resonant Raman process has been considered a potential candidate for use in atomic memories with large bandwidths and high speeds. However, to date, the low memory efficiency remains an unsolved bottleneck. Here, we demonstrate a high-performance atomic Raman memory in Rb87 vapour with the development of an optimal control technique. A memory efficiency of 82.6% for 10-ns optical pulses is achieved and is the highest realized to date in atomic Raman memories. In particular, an unconditional fidelity of up to 98.0%, significantly exceeding the no-cloning limit, is obtained with the tomography reconstruction for a single-photon level coherent input. Our work marks an important advance of atomic Raman memory towards practical applications in quantum information processing.
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