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Optical waveguides made from periodically poled materials provide high confinement of light and enable the generation of new wavelengths via quasi-phase-matching, making them a key platform for nonlinear optics and photonics. However, such devices are not typically employed for high-harmonic generation. Here, using 200-fs, 10-nJ-level pulses of 4100 nm light at 1 MHz, we generate high harmonics up to the 13th harmonic (315 nm) in a chirped, periodically poled lithium niobate (PPLN) waveguide. Total conversion efficiencies into the visible--ultraviolet region are as high as 10 percent. We find that the output spectrum depends on the waveguide poling period, indicating that quasi-phase-matching plays a significant role. In the future, such periodically poled waveguides may enable compact sources of ultrashort pulses at high repetition rates and provide new methods of probing the electronic structure of solid-state materials.
Prospective integrated quantum optical technologies will combine nonlinear optics and components requiring cryogenic operating temperatures. Despite the prevalence of integrated platforms exploiting $chi^{(2)}$-nonlinearities for quantum optics, for
We observe second harmonic generation via random quasi-phase-matching in a 2.0 mu m periodically poled, 1-cm-long, z-cut lithium tantalate. Away from resonance, the harmonic output profiles exhibit a characteristic pattern stemming from a stochastic
Lithium niobate (LN), dubbed by many as the silicon of photonics, has recently risen to the forefront of chip-scale nonlinear optics research since its demonstration as an ultralow-loss integrated photonics platform. Due to its significant quadratic
We report the experimental demonstration of directly produced polarization squeezing at 1064 nm from a type I optical parametric amplifier (OPA) based on a periodically poled KTP crystal (PPKTP). The orthogonal polarization modes of the polarization
We demonstrate enhanced second harmonic generation in a gallium phosphide photonic crystal waveguide with a measured external conversion efficiency of 5$times10^{-7}$/W. Our results are promising for frequency conversion of on-chip integrated emitter