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The Nitrogen-Vacancy (NV) defect in diamond is a unique quantum system that offers precision sensing of nanoscale physical quantities beyond the current state-of-the-art. Here we present a method to controllably encode the interactions in the population of the spin states, thereby introducing a way to control the sensitivity of a single spin as a continuum in contrast to free-evolution based methods. By adopting this feature we demonstrate high-accuracy NV magnetometry without 2pi ambiguities, enhance the dynamic range by a factor of 4*10^3 achieve interaction times exceeding 2 ms in off-the-shelf diamond. We perform nuclear spin-noise spectroscopy in the frequency domain by dynamically controlling the NV spins sensitivity piecewise and in a smooth manner thereby precluding harmonic artefacts and undesired interactions. On a broader perspective dynamical sensitivity control provides an elegant handle on the inherent dynamics of quantum systems, while offering decisive advantages for NV centre applications notably in quantum controls and single molecule NMR/MRI.
Nuclear magnetic resonance (NMR) is a powerful method for determining the structure of molecules and proteins. While conventional NMR requires averaging over large ensembles, recent progress with single-spin quantum sensors has created the prospect o
Understanding the dynamics of a quantum bits environment is essential for the realization of practical systems for quantum information processing and metrology. We use single nitrogen-vacancy (NV) centers in diamond to study the dynamics of a disorde
Manipulation of a quantum system requires the knowledge of how it evolves. To impose that the dynamics of a system becomes a particular target operation (for any preparation of the system), it may be more useful to have an equation of motion for the
A protocol is discussed for preparing a spin chain in a generic many-body state in the asymptotic limit of tailored non-unitary dynamics. The dynamics require the spectral resolution of the target state, optimized coherent pulses, engineered dissipat
Robust, high-fidelity readout is central to quantum device performance. Overcoming poor readout is an increasingly urgent challenge for devices based on solid-state spin defects, particularly given their rapid adoption in quantum sensing, quantum inf