Quantum entanglement is the central resource behind applications in quantum information science, from quantum computers and simulators of complex quantum systems to metrology and secure communication. All of these applications require the quantum control of large networks of quantum bits (qubits) to realize gains and speedups over conventional devices. However, propagating quantum entanglement generally becomes difficult or impossible as the system grows in size, owing to the inevitable decoherence from the complexity of connections between the qubits and increased couplings to the environment. Here, we demonstrate the first step in a modular approach to scaling entanglement by utilizing a hierarchy of quantum buses on a collection of three atomic ion qubits stored in two remote ion trap modules. Entanglement within a module is achieved with deterministic near-field interactions through phonons, and remote entanglement between modules is achieved through a probabilistic interaction through photons. This minimal system allows us to address generic issues in synchronization and scalability of entanglement with multiple buses, while pointing the way toward a modular large-scale quantum computer architecture that promises less spectral crowding and less decoherence. We generate this modular entanglement faster than the observed qubit decoherence rate, thus the system can be scaled to much larger dimensions by adding more modules.