اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدAnomalous Size Dependence of the Thermal Conductivity of Graphene Ribbons
168
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
We investigated the thermal conductivity K of graphene ribbons and graphite slabs as the function of their lateral dimensions. Our theoretical model considered the anharmonic three-phonon processes to the second-order and included the angle-dependent phonon scattering from the ribbon edges. It was found that the long mean free path of the long-wavelength acoustic phonons in graphene can lead to an unusual non-monotonic dependence of the thermal conductivity on the length L of a ribbon. The effect is pronounced for the ribbons with the smooth edges (specularity parameter p>0.5). Our results also suggest that - contrary to what was previously thought - the bulk-like 3D phonons in graphite can make a rather substantial contribution to its in-plane thermal conductivity. The Umklapp-limited thermal conductivity of graphite slabs scales, for L below ~ 10 micrometers, as log(L) while for larger L, the thermal conductivity approaches a finite value following the dependence K_0 - AtimesL^-1/2, where K_0 and A are parameters independent of the length. Our theoretical results clarify the scaling of the phonon thermal conductivity with the lateral sizes in graphene and graphite. The revealed anomalous dependence K(L) for the micrometer-size graphene ribbons can account for some of the discrepancy in reported experimental data for graphene.
قيم البحث
اقرأ أيضاً
Using non-equilibrium molecular dynamics method(NEMD), we have found that the thermal conductivity of multilayer graphene nanoribbons monotonously decreases with the increase of the number of layers, such behavior can be attributed to the phonon reso
nance effect of out-of-plane phonon modes. The reduction of thermal conductivity is found to be proportional to the layer size, which is caused by the increase of phonon resonance. Our results are in agreement with recent experiment on dimensional evolution of thermal conductivity in few layer graphene.
Assuming diffusive carrier transport and employing an effective medium theory, we calculate the temperature dependence of bilayer graphene conductivity due to Fermi-surface broadening as a function of carrier density. We find that the temperature dep
endence of the conductivity depends strongly on the amount of disorder. In the regime relevant to most experiments, the conductivity is a function of T/T*, where T* is the characteristic temperature set by disorder. We demonstrate that experimental data taken from various groups collapse onto a theoretically predicted scaling function.
Graphene is a monolayer of carbon atoms packed into a hexagon lattice to host two pairs of massless two-dimensional Dirac fermions in the absence of or with negligible spin-orbit coupling. It is known that the existence of non-zero electric polarizat
ion in reduced momentum space which is associated with a hidden chiral symmetry will lead to the zero-energy flat band of zigzag nanoribbon. The Adler-Bell-Jackiw chiral anomaly or non-conservation of chiral charges at different valleys can be realized in a confined ribbon of finite width. In the laterally diffusive regime, the finite-size correction to conductivity is always positive and goes inversely with the square of the lateral dimension W, which is different from the finite-size correction inversely with W from boundary modes. This anomalous finite-size conductivity reveals the signature of the chiral anomaly in graphene, and is measurable experimentally.
We address the electronic structure and magnetic properties of vacancies and voids both in graphene and graphene ribbons. Using a mean field Hubbard model, we study the appearance of magnetic textures associated to removing a single atom (vacancy) an
d multiple adjacent atoms (voids) as well as the magnetic interactions between them. A simple set of rules, based upon Lieb theorem, link the atomic structure and the spatial arrangement of the defects to the emerging magnetic order. The total spin $S$ of a given defect depends on its sublattice imbalance, but some defects with S=0 can still have local magnetic moments. The sublattice imbalance also determines whether the defects interact ferromagnetically or antiferromagnetically with one another and the range of these magnetic interactions is studied in some simple cases. We find that in semiconducting armchair ribbons and two-dimensional graphene without global sublattice imbalance there is maximum defect density above which local magnetization disappears. Interestingly, the electronic properties of semiconducting graphene ribbons with uncoupled local moments are very similar to those of diluted magnetic semiconductors, presenting giant Zeeman splitting.
Low-energy Landau levels of AB-stacked zigzag graphene ribbons in the presence of a uniform perpendicular magnetic field (textbf{B}) are investigated by the Peierls coupling tight-binding model. State energies and associated wave functions are domina
ted by the textbf{B}-field strength and the $k_z$-dependent interribbon interactions. The occupied valence bands are asymmetric to the unoccupied conduction bands about the Fermi level. Many doubly degenerate Landau levels and singlet curving magnetobands exist along $k_x$ and $k_z$ directions, respectively. Such features are directly reflected in density of states, which exhibits a lot of asymmetric prominent peaks because of 1D curving bands. The $k_z$-dependent interribbon interactions dramatically modify the magnetobands, such as the lift of double degeneracy, the change of state energies, and the production of two groups of curving magnetobands. They also change the characteristics of the wave functions and cause the redistribution of the charge carrier density. The $k_z$-dependent wave functions are further used to predict the selection rule of the optical transition.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
