The production of $J/psi$ mesons accompanied by open charm, and of pairs of open charm hadrons are observed in pp collisions at a centre-of-mass energy of 7 TeV using an integrated luminosity of $355pb^{-1}$ collected with the LHCb detector. Model independent measurements of absolute cross-sections are given together with ratios to the measured $J/psi$ and open charm cross-sections. The properties of these events are studied and compared to theoretical predictions.