اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدExcitons in Molecular Aggregates with Levy Disorder: Anomalous Localization and Exchange Broadening of Optical Spectra
143
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
We predict the existence of exchange broadening of optical lineshapes in disordered molecular aggregates and a nonuniversal disorder scaling of the localization characteristics of the collective electronic excitations (excitons). These phenomena occur for heavy-tailed Levy disorder distributions with divergent second moments - distributions that play a role in many branches of physics. Our results sharply contrast with aggregate models commonly analyzed, where the second moment is finite. They bear a relevance for other types of collective excitations as well.
قيم البحث
اقرأ أيضاً
The many-body localization transition for Heisenberg spin chain with a speckle disorder is studied. Such a model is equivalent to a system of spinless fermions in an optical lattice with an additional speckle field. Our numerical results show that th
e many-body localization transition in speckle disorder falls within the same universality class as the transition in an uncorrelated random disorder, in contrast to the quasiperiodic potential typically studied in experiments. This hints at possibilities of experimental studies of the role of rare Griffiths regions and of the interplay of ergodic and localized grains at the many-body localization transition. Moreover, the speckle potential allows one to study the role of correlations in disorder on the transition. We study both spectral and dynamical properties of the system focusing on observables that are sensitive to the disorder type and its correlations. In particular, distributions of local imbalance at long times provide an experimentally available tool that reveals the presence of small ergodic grains even deep in the many-body localized phase in a correlated speckle disorder.
Exponential localization of wavefunctions in lattices, whether in real or synthetic dimensions, is a fundamental wave interference phenomenon. Localization of Bloch-type functions in space-periodic lattice, triggered by spatial disorder, is known as
Anderson localization and arrests diffusion of classical particles in disordered potentials. In time-periodic Floquet lattices, exponential localization in a periodically driven quantum system similarly arrests diffusion of its classically chaotic counterpart in the action-angle space. Here we demonstrate that nonlinear optical response allows for clear detection of the disorder-induced phase transition between delocalized and localized states. The optical signature of the transition is the emergence of symmetry-forbidden even-order harmonics: these harmonics are enabled by Anderson-type localization and arise for sufficiently strong disorder even when the overall charge distribution in the field-free system spatially symmetric. The ratio of even to odd harmonic intensities as a function of disorder maps out the phase transition even when the associated changes in the band structure are negligibly small.
We consider heat transport in one-dimensional harmonic chains attached at its ends to Langevin heat baths. The harmonic chain has mass impurities where the separation $d$ between any two successive impurities is randomly distributed according to a po
wer-law distribution $P(d)sim 1/d^{alpha+1}$, being $alpha>0$. In the regime where the first moment of the distribution is well defined ($1<alpha<2$) the thermal conductivity $kappa$ scales with the system size $N$ as $kappasim N^{(alpha-3)/alpha}$ for fixed boundary conditions, whereas for free boundary conditions $kappasim N^{(alpha-1)/alpha}$ if $Ngg1$. When $alpha=2$, the inverse localization length $lambda$ scales with the frequency $omega$ as $lambdasim omega^2 ln omega$ in the low frequency regime, due to the logarithmic correction, the size scaling law of the thermal conductivity acquires a non-closed form. When $alpha>2$, the thermal conductivity scales as in the uncorrelated disorder case. The situation $alpha<1$ is only analyzed numerically, where $lambda(omega)sim omega^{2-alpha}$ which leads to the following asymptotic thermal conductivity: $kappa sim N^{-(alpha+1)/(2-alpha)}$ for fixed boundary conditions and $kappa sim N^{(1-alpha)/(2-alpha)}$ for free boundary conditions.
The quest for nonequilibrium quantum phase transitions is often hampered by the tendency of driving and dissipation to give rise to an effective temperature, resulting in classical behavior. Could this be different when the dissipation is engineered
to drive the system into a nontrivial quantum coherent steady state? In this work we shed light on this issue by studying the effect of disorder on recently-introduced dissipation-induced Chern topological states, and examining the eigenmodes of the Hermitian steady state density matrix or entanglement Hamiltonian. We find that, similarly to equilibrium, each Landau band has a single delocalized level near its center. However, using three different finite size scaling methods we show that the critical exponent $ u$ describing the divergence of the localization length upon approaching the delocalized state is significantly different from equilibrium if disorder is introduced into the non-dissipative part of the dynamics. This indicates a different type of nonequilibrium quantum critical universality class accessible in cold-atom experiments.
Structures with heavy-tailed distributions of disorder occur widely in nature. The evolution of such systems, as in foraging for food or the occurrence of earthquakes is generally analyzed in terms of an incoherent series of events. But the study of
wave propagation or lasing in such systems requires the consideration of coherent scattering. We consider the distribution of wave energy inside 1D random media in which the spacing between scatterers follow a Levy $alpha$-stable distribution characterized by a power-law decay with exponent $alpha$. We show that the averages of the intensity and logarithmic intensity are given in terms of the average of the logarithm of transmission and the depth into the sample raised to the power $alpha$. Mapping the depth into the sample to the number of scattering elements yields intensity statistics that are identical to those found for Anderson localization in standard random media. This allows for the separation for the impacts of disorder distribution and wave coherence in random media.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
