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We demonstrate that a near-dissociation photoassociation resonance can be used to create a deeply bound molecular sample of ultracold NaCs. To probe the resulting vibrational distribution of the sample, we use a new technique that can be applied to any ultracold molecular system. We utilize a tunable pulsed dye laser to produce efficient spectroscopic scans ($sim700$ cm$^{-1}$ at a time) in which we observe the $1^{1} Sigma^{+}rightarrow 2^{1}Sigma^{+}-2^{3}Pi$ vibrational progression, as well as the dissociation limit to the Cs 6$^{2}$P$_{3/2}$ asymptote. We assign $1^{1} Sigma^{+}$$(emph{v}$ = 4, 5, 6, 11, 19) vibrational levels in our sample.
Recently, the quest for an ultracold and dense ensemble of polar molecules has attracted strong interest. Polar molecules have bright prospects for novel quantum gases with long-range and anisotropic interactions, for quantum information science, and
We report the creation of heteronuclear ultralong-range Rydberg-molecule dimers by excitation of minority $^{88}text{Sr}$ atoms to $5sns,^3S_1$ Rydberg states ($n=31-39$) in a dense background of $^{84}text{Sr}$. We observe an isotope shift of the $
This paper reviews the recent results in high-resolution spectroscopy on cold molecules. Laser spectroscopy of cold molecules addresses issues of symmetry violation, like in the search for the electric dipole moment of the electron and the studies on
Aluminum monochloride (AlCl) has been proposed as a promising candidate for laser cooling to ultracold temperatures, and recent spectroscopy results support this prediction. It is challenging to produce large numbers of AlCl molecules because it is a
Ultracold paramagnetic and polar diatomic molecules are among the promising systems for quantum simulation of lattice-spin models. Unfortunately, their experimental observation is still challenging. Based on our recent textit{ab-initio} calculations,