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We examine dark quantum superposition states of weakly bound Rb2 Feshbach molecules and tightly bound triplet Rb2 molecules in the rovibrational ground state, created by subjecting a pure sample of Feshbach molecules in an optical lattice to a bichromatic Raman laser field. We analyze both experimentally and theoretically the creation and dynamics of these dark states. Coherent wavepacket oscillations of deeply bound molecules in lattice sites, as observed in one of our previous experiments, are suppressed due to laser-induced phase locking of molecular levels. This can be understood as the appearance of a novel multilevel dark state. In addition, the experimental methods developed help to determine important properties of our coupled atom / laser system.
Recently, the quest for an ultracold and dense ensemble of polar molecules has attracted strong interest. Polar molecules have bright prospects for novel quantum gases with long-range and anisotropic interactions, for quantum information science, and
We report on the realization of a time-domain `Stuckelberg interferometer, which is based on the internal state structure of ultracold Feshbach molecules. Two subsequent passages through a weak avoided crossing between two different orbital angular m
We report here on the production of an ultracold gas of tightly bound Rb2 molecules in the ro-vibrational triplet ground state, close to quantum degeneracy. This is achieved by optically transferring weakly bound Rb2 molecules to the absolute lowest
We report on the first creation of ultracold bosonic heteronuclear molecules of two fermionic species, 6Li and 40K, by a magnetic field sweep across an interspecies s-wave Feshbach resonance. This allows us to associate up to 4x10^4 molecules with hi
Ultracold paramagnetic and polar diatomic molecules are among the promising systems for quantum simulation of lattice-spin models. Unfortunately, their experimental observation is still challenging. Based on our recent textit{ab-initio} calculations,