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تسجيل مستخدم جديدAnisotropic three-dimensional magnetism in CaFe2As2
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Inelastic neutron scattering measurements on the low energy spin waves in CaFe2As2 show that the magnetic exchange interactions in the Fe layers are exceptionally large and similar to the cuprates. However, the exchange between layers is ~10% of the coupling in the layers and the magnetism is more appropriately categorized as anisotropic three-dimensional, in contrast to the two-dimensional cuprates. Band structure calculations of the spin dynamics and magnetic exchange interactions are in good agreement with the experimental data.
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We use angle-resolved photoemission spectroscopy (ARPES) to study the electronic properties of CaFe2As2 - parent compound of a pnictide superconductor. We find that the structural and magnetic transition is accompanied by a three- to two-dimensional
(3D-2D) crossover in the electronic structure. Above the transition temperature (Ts) Fermi surfaces around Gamma and X points are cylindrical and quasi-2D. Below Ts the former becomes a 3D ellipsoid, while the latter remains quasi-2D. This finding strongly suggests that low dimensionality plays an important role in understanding the superconducting mechanism in pnictides.
Single crystal neutron and high-energy x-ray diffraction have identified the phase lines corresponding to transitions between the ambient-pressure tetragonal (T), the antiferromagnetic orthorhombic (O) and the non-magnetic collapsed tetragonal (cT) p
hases of CaFe2As2. We find no evidence of additional structures for pressures up to 2.5 GPa (at 300 K). Both the T-cT and O-cT transitions exhibit significant hysteresis effects and we demonstrate that coexistence of the O and cT phases can occur if a non-hydrostatic component of pressure is present. Measurements of the magnetic diffraction peaks show no change in the magnetic structure or ordered moment as a function of pressure in the O phase and we find no evidence of magnetic ordering in the cT phase. Band structure calculations show that the transition results in a strong decrease of the iron 3d density of states at the Fermi energy, consistent with a loss of the magnetic moment.
Neutron scattering measurements of the magnetic excitations in single crystals of antiferromagnetic CaFe2As2 reveal steeply dispersive and well-defined spin waves up to an energy of 100 meV. Magnetic excitations above 100 meV and up to the maximum en
ergy of 200 meV are however broader in energy and momentum than the experimental resolution. While the low energy modes can be fit to a Heisenberg model, the total spectrum cannot be described as arising from excitations of a local moment system. Ab-initio calculations of the dynamic magnetic susceptibility suggest that the high energy behavior is dominated by the damping of spin waves by particle-hole excitations.
Aliovalent rare earth substitution into the alkaline earth site of CaFe2As2 single-crystals is used to fine-tune structural, magnetic and electronic properties of this iron-based superconducting system. Neutron and single crystal x-ray scattering exp
eriments indicate that an isostructural collapse of the tetragonal unit cell can be controllably induced at ambient pressures by choice of substituent ion size. This instability is driven by the interlayer As-As anion separation, resulting in an unprecedented thermal expansion coefficient of $180times 10^{-6}$ K$^{-1}$. Electrical transport and magnetic susceptibility measurements reveal abrupt changes in the physical properties through the collapse as a function of temperature, including a reconstruction of the electronic structure. Superconductivity with onset transition temperatures as high as 47 K is stabilized by the suppression of antiferromagnetic order via chemical pressure, electron doping or a combination of both. Extensive investigations are performed to understand the observations of partial volume-fraction diamagnetic screening, ruling out extrinsic sources such as strain mechanisms, surface states or foreign phases as the cause of this superconducting phase that appears to be stable in both collapsed and uncollapsed structures.
Interplay between antiferromagnetism and superconductivity is studied by using the 3-dimensional nearly half-filled Hubbard model with anisotropic transfer matrices $t_{rm z}$ and $t_{perp}$. The phase diagrams are calculated for varying values of th
e ratio $r_{rm z}=t_{rm z}/t_{perp}$ using the spin fluctuation theory within the fluctuation-exchange approximation. The antiferromagnetic phase around the half-filled electron density expands while the neighboring phase of the anisotropic $d_{x^{2}-y^{2}}$-wave superconductivity shrinks with increasing $r_{rm z}$. For small $r_{rm z}$ $T_{rm c}$ decreases slowly with increasing $r_{rm z}$. For moderate values of $r_{rm z}$ we find the second order transition, with lowering temperature, from the $d_{x^{2}-y^{2}}$-wave superconducting phase to a phase where incommensurate SDW coexists with $d_{x^{2}-y^{2}}$-wave superconductivity. Resonance peaks as were discussed previously for 2D superconductors are shown to survive in the $d_{x^{2}-y^{2}}$-wave superconducting phase of 3D systems. Soft components of the incommensurate SDW spin fluctuation mode grow as the coexistent phase is approached.
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